Evidence map›Paper›PMID 38459235›Full record

ArticleNature chemistry2024

Reconfiguring hydrogel assemblies using a photocontrolled metallopolymer adhesive for multiple customized functions.

Jiahui Liu, Yun-Shuai Huang, Yazhi Liu, Dachuan Zhang, Kaloian Koynov, Hans-Jürgen Butt, Si Wu

Abstract read
In one paragraph

Article in Nature chemistry, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 34 papers.

0numbers the graph read from it
0cells of the map it votes in
34citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

34 citing papers in PubMed.

  1. Review
  2. Article
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  7. Recyclable Photopolymers for Sustainable 3D Printing.Polymer science & technology (Washington, D.C.) · 2026
    Review
  8. Article
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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

7 authors.

Jiahui LiuHefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Anhui Key Laboratory of Optoelectronic Science and Technology, Department of Polymer Science and Engineering, University of Science and Technology of China, Hefei, China.
Yun-Shuai HuangHefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Anhui Key Laboratory of Optoelectronic Science and Technology, Department of Polymer Science and Engineering, University of Science and Technology of China, Hefei, China.
Yazhi LiuHefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Anhui Key Laboratory of Optoelectronic Science and Technology, Department of Polymer Science and Engineering, University of Science and Technology of China, Hefei, China.
Dachuan ZhangHefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Anhui Key Laboratory of Optoelectronic Science and Technology, Department of Polymer Science and Engineering, University of Science and Technology of China, Hefei, China.
Kaloian KoynovMax Planck Institute for Polymer Research, Mainz, Germany.ORCID http://orcid.org/0000-0002-4062-8834
Hans-Jürgen ButtMax Planck Institute for Polymer Research, Mainz, Germany.ORCID http://orcid.org/0000-0001-5391-2618
Si WuHefei National Research Center for Physical Sciences at the Microscale, CAS Key Laboratory of Soft Matter Chemistry, Anhui Key Laboratory of Optoelectronic Science and Technology, Department of Polymer Science and Engineering, University of Science and Technology of China, Hefei, China. siwu@ustc.edu.cn.ORCID http://orcid.org/0000-0001-8156-346X

Funding

National Natural Science Foundation of China (National Science Foundation of China) 52073268National Natural Science Foundation of China (National Science Foundation of China) 52120105004Natural Science Foundation of Anhui Province (Anhui Provincial Natural Science Foundation) 1908085MB38
6 · The paper itself

Abstract

Stimuli-responsive hydrogels with programmable shape changes are promising materials for soft robots, four-dimensional printing, biomedical devices and artificial intelligence systems. However, these applications require the fabrication of hydrogels with complex, heterogeneous and reconfigurable structures and customizable functions. Here we report the fabrication of hydrogel assemblies with these features by reversibly gluing hydrogel units using a photocontrolled metallopolymer adhesive. The metallopolymer adhesive firmly attached individual hydrogel units via metal-ligand coordination and polymer chain entanglement. Hydrogel assemblies containing temperature- and pH-responsive hydrogel units showed controllable shape changes and motions in response to these external stimuli. To reconfigure their structures, the hydrogel assemblies were disassembled by irradiating the metallopolymer adhesive with light; the disassembled hydrogel units were then reassembled using the metallopolymer adhesive with heating. The shape change and structure reconfiguration abilities allow us to reprogramme the functions of hydrogel assemblies. The development of reconfigurable hydrogel assemblies using reversible adhesives provides a strategy for designing intelligent materials and soft robots with user-defined functions.

Identifiers

PMID38459235
PMCPMC11164683

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.