Evidence map›Paper›PMID 38437562›Full record

ArticleProceedings of the National Academy of Sciences of the United States of America2024

Chelation-directed interface engineering of in-place self-cleaning membranes.

Xiaobin Yang, Yangxue Li, Dan Wu, Linlin Yan, Jingzhu Guan, Yajie Wen, Yongping Bai, Bhekie B Mamba, Seth B Darling, Lu Shao

Open access · hybridAbstract read
In one paragraph

Article in Proceedings of the National Academy of Sciences of the United States of America, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers, 1 of them a synthesis that pooled it.

0numbers the graph read from it
0cells of the map it votes in
6citing papers in PubMed, 1 pooled it
7.9field-weighted citation impact, top 2% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

6 citing papers in PubMed, 1 synthesis or guideline pooled it, 39 citations in OpenAlex.

  1. Pooled it
  2. Review
  3. Article
  4. Article
  5. Review
  6. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

10 authors at 3 institutions in 3 countries.

Xiaobin YangMinistry of Industry and Information Technology Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, People's Republic of China.ORCID 0009-0004-5431-730X
Yangxue LiMinistry of Industry and Information Technology Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, People's Republic of China.
Dan WuLongjiang Environmental Protection Group CO., LTD, Harbin 150050, People's Republic of China.
Linlin YanSchool of Marine Science and Technology, State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology, Weihai 264209, People's Republic of China.
Jingzhu GuanMinistry of Industry and Information Technology Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, People's Republic of China.
Yajie WenMinistry of Industry and Information Technology Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, People's Republic of China.
Yongping BaiMinistry of Industry and Information Technology Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, People's Republic of China.
Bhekie B MambaInstitute for Nanotechnology and Water Sustainability, College of Engineering, Science and Technology, University of South Africa, Roodepoort 1709, South Africa.
Seth B DarlingChemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, IL 60439.ORCID 0000-0002-5461-6965
Lu ShaoMinistry of Industry and Information Technology Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage, State Key Laboratory of Urban Water Resource and Environment, School of Chemistry and Chemical Engineering, Harbin Institute of Technology, Harbin 150001, People's Republic of China.ORCID 0000-0002-4161-3861
Harbin Institute of Technology · CNArgonne National Laboratory · USUniversity of South Africa · ZA

Funding

DOE | SC | Basic Energy Sciences (BES) AMEWS EFRCHeilongjiang Touyan Team HITTY-20190033National Natural Science Foundation of China 22178076 22111530113Natural Science Foundation of Heilongjiang Province for Distinguished Young Scholars JQ2020B001
6 · The paper itself

Abstract

Water-energy sustainability will depend upon the rapid development of advanced pressure-driven separation membranes. Although energy-efficient, water-treatment membranes are constrained by ubiquitous fouling, which may be alleviated by engineering self-cleaning membrane interfaces. In this study, a metal-polyphenol network was designed to direct the armorization of catalytic nanofilms (ca. 18 nm) on inert polymeric membranes. The chelation-directed mineralized coating exhibits high polarity, superhydrophilicity, and ultralow adhesion to crude oil, enabling cyclable crude oil-in-water emulsion separation. The in-place flux recovery rate exceeded 99.9%, alleviating the need for traditional ex situ cleaning. The chelation-directed nanoarmored membrane exhibited 48-fold and 6.8-fold figures of merit for in-place self-cleaning regeneration compared to the control membrane and simple hydraulic cleaning, respectively. Precursor interaction mechanisms were identified by density functional theory calculations. Chelation-directed armorization offers promise for sustainable applications in catalysis, biomedicine, environmental remediation, and beyond.

Indexed as

catalytic self-cleaningchelationmembraneoil separationwater treatment

Identifiers

PMID38437562
PMCPMC10945774
OpenAlexW4392367144

What OpenQuestion holds

Textmetadata
LicenceCC BY-NC-ND
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.