ArticleNature nanotechnology2024
Complete miscibility of immiscible elements at the nanometre scale.
Article in Nature nanotechnology, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
What it found
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Who cites it
12 citing papers in PubMed.
- Universal synthesis of high-entropy alloy nanostructures with femtosecond lasers.Science advances · 2026Article
- Polyelemental Nanoparticle Catalysts.Advanced materials (Deerfield Beach, Fla.) · 2026Review
- Self-adhesive high-entropy oxide sub-nanowire monolithic electrocatalysts.Nature nanotechnology · 2026Article
- Structure Inhomogeneity of Gold Nanoparticles and Its Effect on HNanomaterials (Basel, Switzerland) · 2026Article
- Oxidation-resistant AgRuIr alloy nanocages for efficient and enduring oxygen evolution in proton exchange membrane electrolysis.Nature communications · 2026Article
- Kinetically Controlling Surface Atom Arrangements in Thermally Robust, Amorphous High-Entropy Alloy Nanoparticles by Solvent Selection.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Phase Formation of Multielement Nanoparticles from Immiscible Elements in Electrically Exploding Joint-Twisted Wires.Nanomaterials (Basel, Switzerland) · 2025Article
- High-throughput design of bimetallic materialsChemical science · 2025Article
- Polyelemental Nanoparticle Synthesis Enabled by Noncontact Metallothermic Reactions.Journal of the American Chemical Society · 2025Article
- An integrated AI-driven framework for maximizing the efficiency of heterostructured nanomaterials in photocatalytic hydrogen production.Scientific reports · 2025Article
- Gold Decoration To Improve Rh-Nanoalloys for CO-Adsorption.The journal of physical chemistry. C, Nanomaterials and interfaces · 2025Article
- Airborne metal nanoparticles released by azides detonation: determination and potential public exposure.Scientific reports · 2024Article
Corrections and comments
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Authors and funding
9 authors.
Funding
Abstract
Understanding the mixing behaviour of elements in a multielement material is important to control its structure and property. When the size of a multielement material is decreased to the nanoscale, the miscibility of elements in the nanomaterial often changes from its bulk counterpart. However, there is a lack of comprehensive and quantitative experimental insight into this process. Here we explored how the miscibility of Au and Rh evolves in nanoparticles of sizes varying from 4 to 1 nm and composition changing from 15% Au to 85% Au. We found that the two immiscible elements exhibit a phase-separation-to-alloy transition in nanoparticles with decreased size and become completely miscible in sub-2 nm particles across the entire compositional range. Quantitative electron microscopy analysis and theoretical calculations were used to show that the observed immiscibility-to-miscibility transition is dictated by particle size, composition and possible surface adsorbates present under the synthesis conditions.
Identifiers
38429491What OpenQuestion holds
Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.