ArticleJACS Au2024
Role of the Benzothiadiazole Unit in Organic Polymers on Photocatalytic Hydrogen Production.
Article in JACS Au, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed, 18 citations in OpenAlex.
- Residual metal single-atom catalysis: enhanced photocatalytic hydrogen productionChemical science · 2026Article
- Design strategies, methods, and photophysical insights in polymeric photocatalysts for solar-driven hydrogen evolution.Nano convergence · 2026Review
- Highly Efficient Platinum-Free Photocatalytic Hydrogen Evolution From Low-cost Conjugated Polymer Nanoparticles.Advanced materials (Deerfield Beach, Fla.) · 2025Article
- Molecular Dipole Buffer Layer Enabling Compact Interfaces in Perovskite Solar Cells.ACS energy letters · 2025Article
- High-Throughput Screening of Molecule/Polymer Photocatalysts for the Hydrogen Evolution Reaction.ACS catalysis · 2025Article
- Covalently linked molecular catalysts in conjugated polymer dots boost photocatalytic alcohol oxidation in neutral condition.Nature communications · 2024Article
- Hydrophilic Photocrosslinkers as a Universal Solution to Endow Water Affinity to a Polymer Photocatalyst for an Enhanced Hydrogen Evolution Rate.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
Corrections and comments
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Authors and funding
5 authors at 2 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Organic polymers based on the donor-acceptor structure are a promising class of efficient photocatalysts for solar fuel production. Among these polymers, poly(9,9-dioctylfluorene-alt-1,2,3-benzothiadiazole) (PFBT) consisting of fluorene donor and benzothiadiazole acceptor units has shown good photocatalytic activity when it is prepared into polymer dots (Pdots) in water. In this work, we investigate the effect of the chemical environment on the activity of photocatalysis from PFBT Pdots for hydrogen production. This is carried out by comparing the samples with various concentrations of palladium under different pH conditions and with different sacrificial electron donors (SDs). Moreover, a model compound 1,2,3-benzothiadiazole di-9,9-dioctylfluorene (BTDF) is synthesized to investigate the mechanism for protonation of benzothiadiazole and its kinetics in the presence of an organic acid-salicylic acid by cyclic voltammetry. We experimentally show that benzothiadiazole in BTDF can rapidly react with protons with a fitted value of 0.1-5 × 10
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Registered trials
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