Evidence map›Paper›PMID 38413812›Full record

ArticleNature materials2024

High-density stable glasses formed on soft substrates.

Peng Luo, Sarah E Wolf, Shivajee Govind, Richard B Stephens, Dong Hyup Kim, Cindy Y Chen, Truc Nguyen, Patryk Wąsik, Mikhail Zhernenkov, Brandon Mcclimon and 1 more

Open access · greenAbstract read
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In one paragraph

Article in Nature materials, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.

0numbers the graph read from it
0cells of the map it votes in
4citing papers in PubMed
3.9field-weighted citation impact, top 3% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

4 citing papers in PubMed, 33 citations in OpenAlex.

  1. Article
  2. Article
  3. Article
  4. Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

11 authors at 4 institutions in 2 countries.

Peng LuoDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA, USA.ORCID http://orcid.org/0000-0003-4280-4990
Sarah E WolfDepartment of Chemistry, State University of New York Cortland, Cortland, NY, USA.ORCID http://orcid.org/0000-0001-7695-7923
Shivajee GovindDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA, USA.ORCID http://orcid.org/0000-0003-2356-4063
Richard B StephensDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA, USA.ORCID http://orcid.org/0000-0002-7034-6141
Dong Hyup KimDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA, USA.ORCID http://orcid.org/0000-0003-3866-1878
Cindy Y ChenDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA, USA.ORCID http://orcid.org/0000-0001-7401-3638
Truc NguyenDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA, USA.
Patryk WąsikNational Synchrotron Light Source II (NSLS-II), Brookhaven National Laboratory, Upton, NY, USA.ORCID http://orcid.org/0000-0002-7447-7472
Mikhail ZhernenkovNational Synchrotron Light Source II (NSLS-II), Brookhaven National Laboratory, Upton, NY, USA.
Brandon McclimonDepartment of Mechanical Engineering and Applied Mechanics, University of Pennsylvania, Philadelphia, PA, USA.ORCID http://orcid.org/0000-0002-2163-7495
Zahra FakhraaiDepartment of Chemistry, University of Pennsylvania, Philadelphia, PA, USA. fakhraai@sas.upenn.edu.ORCID http://orcid.org/0000-0002-0597-9882
University of Pennsylvania · USBrookhaven National Laboratory · USSeoul National University · KRSUNY Cortland · US

Funding

National Science Foundation (NSF) DGE-1845298National Science Foundation (NSF) DMR-1720530
6 · The paper itself

Abstract

Enabled by surface-mediated equilibration, physical vapour deposition can create high-density stable glasses comparable with liquid-quenched glasses aged for millions of years. Deposition is often performed at various rates and temperatures on rigid substrates to control the glass properties. Here we demonstrate that on soft, rubbery substrates, surface-mediated equilibration is enhanced up to 170 nm away from the interface, forming stable glasses with densities up to 2.5% higher than liquid-quenched glasses within 2.5 h of deposition. Gaining similar properties on rigid substrates would require 10 million times slower deposition, taking ~3,000 years. Controlling the modulus of the rubbery substrate provides control over the glass structure and density at constant deposition conditions. These results underscore the significance of substrate elasticity in manipulating the properties of the mobile surface layer and thus the glass structure and properties, allowing access to deeper states of the energy landscape without prohibitively slow deposition rates.

Identifiers

PMID38413812
OpenAlexW4392192993

What OpenQuestion holds

Textmetadata
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.