ArticleProceedings of the National Academy of Sciences of the United States of America2024
A universal and scalable transformation of bulk metals into single-atom catalysts in ionic liquids.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.
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3 citing papers in PubMed, 6 citations in OpenAlex.
- Linking Synthetic Materials Chemistry to Electrocatalytic Performance.Angewandte Chemie (International ed. in English) · 2026Review
- Scalable and Customizable Single-Atom Coatings for pH-Universal HAdvanced materials (Deerfield Beach, Fla.) · 2026Article
- Unleashing the potential of Li-OChemical science · 2024Article
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16 authors at 5 institutions in 2 countries.
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Abstract
Single-atom catalysts (SACs) with maximized metal atom utilization and intriguing properties are of utmost importance for energy conversion and catalysis science. However, the lack of a straightforward and scalable synthesis strategy of SACs on diverse support materials remains the bottleneck for their large-scale industrial applications. Herein, we report a general approach to directly transform bulk metals into single atoms through the precise control of the electrodissolution-electrodeposition kinetics in ionic liquids and demonstrate the successful applicability of up to twenty different monometallic SACs and one multimetallic SAC with five distinct elements. As a case study, the atomically dispersed Pt was electrodeposited onto Ni
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