ArticleScience advances2024
Compact realization of all-attosecond pump-probe spectroscopy.
Article in Science advances, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed, 34 citations in OpenAlex.
- Table-top all-attosecond transient absorption spectroscopy.Nature communications · 2026Article
- Redirection and reshaping of intense extreme-ultraviolet radiation.Science advances · 2026Article
- Coherent control of electron-ion entanglement in multiphoton ionization.Light, science & applications · 2026Article
- High gas-pressure apparatus for nonlinear X-ray propagation and reshaping via stimulated X-ray Raman scattering.Scientific reports · 2025Article
- The Quantum Information Science Challenge for Chemistry.The journal of physical chemistry letters · 2025Review
- Ultrafast energy-dispersive soft-x-ray diffraction in the water window with a laser-driven source.Structural dynamics (Melville, N.Y.) · 2024Article
- Isolated attosecond pulse generation in a semi-infinite gas cell driven by time-gated phase matching.Light, science & applications · 2024Article
Corrections and comments
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Authors and funding
7 authors at 1 institution in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The ability to perform attosecond-pump attosecond-probe spectroscopy (APAPS) is a longstanding goal in ultrafast science. While first pioneering experiments demonstrated the feasibility of APAPS, the low repetition rates (10 to 120 Hz) and the large footprints of existing setups have so far hindered the widespread exploitation of APAPS. Here, we demonstrate two-color APAPS using a commercial laser system at 1 kHz, straightforward post-compression in a hollow-core fiber, and a compact high-harmonic generation (HHG) setup. The latter enables the generation of intense extreme-ultraviolet (XUV) pulses by using an out-of-focus HHG geometry and by exploiting a transient blueshift of the driving laser in the HHG medium. Near-isolated attosecond pulses are generated, as demonstrated by one-color and two-color XUV-pump XUV-probe experiments. Our concept allows selective pumping and probing on extremely short timescales in many laboratories and permits investigations of fundamental processes that are not accessible by other pump-probe techniques.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.