ArticleNature communications2024
In-situ formatting donor-acceptor polymer with giant dipole moment and ultrafast exciton separation.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
What it found
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Who cites it
12 citing papers in PubMed.
- Activating Triplet Excitons in COFs via Layer-Bridging Co Single Atoms for Photocatalytic HAngewandte Chemie (International ed. in English) · 2026Article
- Photo-assisted Rechargeable Organic Batteries: Principle, Advancements, and Perspectives.ChemSusChem · 2026Review
- Ultrafast energy transfer across Pd/MXene interface via hot phonon-electron interactions.Science advances · 2026Article
- Single-atom photocatalyst for click reaction.Nature communications · 2026Article
- Phosphorus and boron enhanced N-doped carbon nanofibers for enhanced lithium ion storage.RSC advances · 2025Article
- Article
- Charge-transfer dynamics in S-scheme photocatalyst.Nature reviews. Chemistry · 2025Review
- Review
- Nanoconfinement Effects in Electrocatalysis and Photocatalysis.Small (Weinheim an der Bergstrasse, Germany) · 2025Review
- Fine-tuning d-p hybridization in Ni-BNature communications · 2025Article
- Electric Fields in Polymeric Systems.Chemical reviews · 2024Review
- A superlattice interface and S-scheme heterojunction for ultrafast charge separation and transfer in photocatalytic HNature communications · 2024Article
Corrections and comments
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Authors and funding
7 authors.
Funding
Abstract
Donor-acceptor semiconducting polymers present countless opportunities for application in photocatalysis. Previous studies have showcased their advantages through direct bottom-up methods. Unfortunately, these approaches often involve harsh reaction conditions, overlooking the impact of uncontrolled polymerization degrees on photocatalysis. Besides, the mechanism behind the separation of electron-hole pairs (excitons) in donor-acceptor polymers remains elusive. This study presents a post-synthetic method involving the light-induced transformation of the building blocks of hyper-cross-linked polymers from donor-carbon-donor to donor-carbon-acceptor states, resulting in a polymer with a substantial intramolecular dipole moment. Thus, excitons are efficiently separated in the transformed polymer. The utility of this strategy is exemplified by the enhanced photocatalytic hydrogen peroxide synthesis. Encouragingly, our observations reveal the formation of intramolecular charge transfer states using time-resolved techniques, confirming transient exciton behavior involving separation and relaxation. This light-induced method not only guides the development of highly efficient donor-acceptor polymer photocatalysts but also applies to various fields, including organic solar cells, light-emitting diodes, and sensors.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.