ArticleNature communications2024
Unified picture of vibrational relaxation of OH stretch at the air/water interface.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
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Who cites it
11 citing papers in PubMed.
- Hydrogen bonding in water under extreme confinement.Nature · 2026Article
- The Origin of the Frequency-Dependence of OH Stretch Vibrational Lifetimes in Liquid Water.The journal of physical chemistry letters · 2026Article
- Inhomogeneity and Vibrational Coupling of Free OH Stretch at the Air/Water Interface.Journal of the American Chemical Society · 2026Article
- The importance of layer-dependent molecular twisting for the structural anisotropy of interfacial water.Science advances · 2026Article
- Alkaline electrocatalytic water oxidation by Fe-Ni nanostructures on porous turbostratic carbon with tailorable metal-metal active sites.Chemical science · 2026Article
- Electric fields at hydrophobic water interfaces: spectroscopic evidence, physical origin, and implications on reactivity.Chemical Society reviews · 2026Review
- Water Under Molecular Crowding: From Femtosecond H-Bond Networks Dynamics to Biological Function.Sub-cellular biochemistry · 2026Review
- Probing catalyst-free hydroxyl radical generation at microbubble interfaces.Nature communications · 2025Article
- Rapid identification platform of spores based on Raman spectroscopy.Food chemistry: X · 2025Article
- Article
- Frequency-Dependent Vibrational Relaxation Time of OH Stretch at the Air/Isotopically Diluted Water Interface.The journal of physical chemistry letters · 2025Article
Corrections and comments
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Authors and funding
4 authors.
Funding
Abstract
The elucidation of the energy dissipation process is crucial for understanding various phenomena occurring in nature. Yet, the vibrational relaxation and its timescale at the water interface, where the hydrogen-bonding network is truncated, are not well understood and are still under debate. In the present study, we focus on the OH stretch of interfacial water at the air/water interface and investigate its vibrational relaxation by femtosecond time-resolved, heterodyne-detected vibrational sum-frequency generation (TR-HD-VSFG) spectroscopy. The temporal change of the vibrationally excited hydrogen-bonded (HB) OH stretch band (ν=1→2 transition) is measured, enabling us to determine reliable vibrational relaxation (T
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Registered trials
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