ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2024
Mechanical Stretch α-Cyclodextrin Pseudopolyrotaxane Elastomer with Reversible Phosphorescence Behavior.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed, 35 citations in OpenAlex.
- Resonator-based add-drop filters enabled by flexible polymorphic crystals with TADF-RTP motifs.Chemical science · 2026Article
- Sensitive mechanical compression-patterned phosphorescence in the rubbery state of cross-linked polymer network.Nature communications · 2025Article
- Full-color programmable high temperature afterglow polymers based on single-molecule emitters.Nature communications · 2025Article
- Highly efficient ionic actuators enabled by sliding ring molecule actuation.Nature communications · 2025Article
- Synthesis of supramolecular polymers with calix[4]arene and β-cyclodextrin and their application in heavy metal ion absorption.RSC advances · 2024Article
- Mechanical Stretch α-Cyclodextrin Pseudopolyrotaxane Elastomer with Reversible Phosphorescence Behavior.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Monomeric, Oligomeric, Polymeric, and Supramolecular Cyclodextrins as Catalysts for Green Chemistry.Research (Washington, D.C.) · 2024Article
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Authors and funding
5 authors at 1 institution in 1 country.
Funding
Abstract
Polyethylene glycol chains in two terminals of the naphthalene functional group are threaded into α-cyclodextrin cavities to form the pseudopolyrotaxane (NPR), which not only effectively induces the phosphorescence of the naphthalene functional group by the cyclodextrin macrocycle confinement, but also provides interfacial hydrogen bonding assembly function between polyhydroxy groups of cyclodextrin and waterborne polyurethane (WPU) chains to construct elastomers. The introduction of NPR endows the elastomer with enhanced mechanical properties and excellent room temperature phosphorescent (RTP) emission (phosphorescence remains in water, acid, alkali, and organic solvents, even at 160 °C high temperatures). Especially, the reversible mechanically responsive room temperature phosphorescence behavior (phosphorescence intensity increased three times under 200% strain) can be observed in the mechanical stretch and recover process, owing to strain-induced microstructural changes further inhibiting the non-radiative transition and the vibration of NPR. Therefore, changing the phosphorescence behavior of supramolecular elastomers through mechanical stretching provides a new approach for supramolecular luminescent materials.
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Registered trials
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