Evidence map›Paper›PMID 38260621›Full record

ArticleResearch square2024

Light-driven C-H activation mediated by 2D transition metal dichalcogenides.

Jingang Li, Di Zhang, Zhongyuan Guo, Xi Jiang, Jonathan M Larson, Haoyue Zhu, Tianyi Zhang, Yuqian Gu, Brian Blankenship, Min Chen and 10 more

Abstract readPreprint
PubMed Full text at PMC Publisher
In one paragraph

Article in Research square, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.

0numbers the graph read from it
0cells of the map it votes in
0citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

0 citing papers in PubMed.

No citing paper in PubMed yet.

4 · The record

Corrections and comments

5 · Who and what money

Authors and funding

20 authors.

Jingang LiMaterials Science & Engineering Program, Texas Materials Institute, and Walker Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX 78712, USA.ORCID 0000-0003-0827-9758
Di ZhangAdvanced Institute for Materials Research (WPI-AIMR), Tohoku University, Sendai 980-8577, Japan.
Zhongyuan GuoAdvanced Institute for Materials Research (WPI-AIMR), Tohoku University, Sendai 980-8577, Japan.ORCID 0000-0003-2406-3877
Xi JiangMaterials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.
Jonathan M LarsonDepartment of Chemistry and Biochemistry, Baylor University, Waco, TX 76798, USA.ORCID 0000-0002-5389-0794
Haoyue ZhuDepartment of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA.
Tianyi ZhangDepartment of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA.
Yuqian GuChandra Family Department of Electrical & Computer Engineering, The University of Texas at Austin, Austin, TX 78712, USA.
Brian BlankenshipLaser Thermal Laboratory, Department of Mechanical Engineering, University of California, Berkeley, CA 94720, USA.
Min ChenDepartment of Materials Science and Engineering, University of California, Berkeley, CA 94720, USA.
Zilong WuMaterials Science & Engineering Program, Texas Materials Institute, and Walker Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX 78712, USA.
Suichu HuangMaterials Science & Engineering Program, Texas Materials Institute, and Walker Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX 78712, USA.
Robert KosteckiEnergy Storage and Distributed Resources Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA.ORCID 0000-0002-4014-8232
Andrew M MinorDepartment of Materials Science and Engineering, University of California, Berkeley, CA 94720, USA.ORCID 0000-0003-3606-8309
Costas P GrigoropoulosLaser Thermal Laboratory, Department of Mechanical Engineering, University of California, Berkeley, CA 94720, USA.ORCID 0000-0002-8505-4037
Deji AkinwandeChandra Family Department of Electrical & Computer Engineering, The University of Texas at Austin, Austin, TX 78712, USA.ORCID 0000-0001-7133-5586
Mauricio TerronesDepartment of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA.
Joan M RedwingDepartment of Materials Science and Engineering, The Pennsylvania State University, University Park, PA 16802, USA.ORCID 0000-0002-7906-452X
Hao LiAdvanced Institute for Materials Research (WPI-AIMR), Tohoku University, Sendai 980-8577, Japan.ORCID 0000-0002-7577-1366
Yuebing ZhengMaterials Science & Engineering Program, Texas Materials Institute, and Walker Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX 78712, USA.ORCID 0000-0002-9168-9477

Funding

On-Chip Multiplexed Adhesion Frequency Assay for Measuring Receptor-Ligand Interactions on CellsDP2GM128446 · NIGMS · UNIVERSITY OF TEXAS AT AUSTIN · PI ZHENG, YUEBING · 2017 to 2017
$2.2M
NIGMS NIH HHS DP2 GM128446
6 · The paper itself

Abstract

C-H bond activation enables the facile synthesis of new chemicals. While C-H activation in short-chain alkanes has been widely investigated, it remains largely unexplored for long-chain organic molecules. Here, we report light-driven C-H activation in complex organic materials mediated by 2D transition metal dichalcogenides (TMDCs) and the resultant solid-state synthesis of luminescent carbon dots in a spatially-resolved fashion. We unravel the efficient H adsorption and a lowered energy barrier of C-C coupling mediated by 2D TMDCs to promote C-H activation. Our results shed light on 2D materials for C-H activation in organic compounds for applications in organic chemistry, environmental remediation, and photonic materials.

Identifiers

PMID38260621
PMCPMC10802730

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.