ArticleNature communications2024
Site-specific metal-support interaction to switch the activity of Ir single atoms for oxygen evolution reaction.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 27 papers, 1 of them a synthesis that pooled it.
What it found
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The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
27 citing papers in PubMed, 1 synthesis or guideline pooled it.
- Precision Design of Single-Atom Catalysts for High-Performance Biosensors.Chemical record (New York, N.Y.) · 2026Pooled it
- Nanocluster-Assisted OH Ligand Modification Optimizes Activity and Stability of Fe-N-C Catalysts.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Unveiling the Structure-Performance Relationship in Ruthenium-Based Anode Catalysts for PEM Water Electrolyzers.Small methods · 2026Review
- Coordination Engineering of Ir─Mo Atomic Pair Sites to Break Scaling Limitations for Acidic Oxygen Evolution.Angewandte Chemie (International ed. in English) · 2026Article
- Single-Atom Catalysts (SACs) for High-Efficiency Water Electrolysis: A Comprehensive Review.Materials (Basel, Switzerland) · 2026Review
- Metal-support interactionsChemical science · 2026Review
- Scalable microfluidic synthesis of noble metal single-atom catalysts.National science review · 2026Article
- Tuning and Shielding Iridium Active Sites Through Tungsten Electron Buffer for Oxygen Evolution Catalysis.Angewandte Chemie (International ed. in English) · 2026Article
- Site-Specific Ir Single Atoms in Spinel Induce 5d Spin Polarization for Enhanced Oxygen Evolution.Angewandte Chemie (International ed. in English) · 2026Article
- Engineering of Asymmetric Dual-Atom Sites for Effective Oxygen Electrocatalysis.Nano-micro letters · 2026Review
- Oxygen Evolution Reaction Catalysts for Acidic-Media COAdvanced materials (Deerfield Beach, Fla.) · 2026Review
- Article
- Atomic-level bonding inducing strong metal-support interaction.National science review · 2025Article
- Durable acidic water oxidation ruthenium based electrocatalyst by fluorination induced symmetry breaking.Nature communications · 2025Article
- Facile Synthesis of High Areal Density and Stable Pt Single-Atom Electrocatalysts by Arc Discharge Atomization and CoNi Trapping.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Spin-polarized Acidic Water Electrolysis with Antenna-Reactor Plasmonic Electrocatalysts.Advanced materials (Deerfield Beach, Fla.) · 2025Article
- Asymmetric coordination enhances the synergy of Pt species dual active sites for efficient photocatalytic HNature communications · 2025Article
- Single-Atom Nano-Islands: Unlocking New Horizons in Catalytic Activity and Stability.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- Polymer-guided grafting of single W atoms onto titanate nanotubes increases SERS activity in semiconductors.Nature communications · 2025Article
- Atomic-scale self-rearrangement of hetero-metastable phases into high-density single-atom catalysts for the oxygen evolution reaction.Nature communications · 2025Article
Corrections and comments
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Authors and funding
10 authors.
Funding
Abstract
The metal-support interactions (MSI) could greatly determine the electronic properties of single-atom catalysts, thus affecting the catalytic performance. However, the typical approach to regulating MSI usually suffers from interference of the variation of supports or sacrificing the stability of catalysts. Here, we effectively regulate the site-specific MSI of Ir single atoms anchored on Ni layered double hydroxide through an electrochemical deposition strategy. Cathodic deposition drives Ir atoms to locate at three-fold facial center cubic hollow sites with strong MSI, while anodic deposition drives Ir atoms to deposit onto oxygen vacancy sites with weak MSI. The mass activity and intrinsic activity of Ir single-atom catalysts with strong MSI towards oxygen evolution reaction are 19.5 and 5.2 times that with weak MSI, respectively. Mechanism study reveals that the strong MSI between Ir atoms and the support stimulates the activity of Ir sites by inducing the switch of active sites from Ni sites to Ir sites and optimizes the adsorption strength of intermediates, thereby enhancing the activity.
Identifiers
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.