ArticleNature communications2024
Oxophilic Ce single atoms-triggered active sites reverse for superior alkaline hydrogen evolution.
Article in Nature communications, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
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Who cites it
9 citing papers in PubMed.
- Zeolitic isolated protonic acid sites-mediated NHNature communications · 2026Article
- Atomically dispersed Ce species adjacent to Ni nanoparticles as hydrogen scavengers for efficient catalytic ammonia decomposition.Nature communications · 2026Article
- Frontier-orbital modulation of rhodium single-atom catalysts for enhanced hydrogen evolution.Nature communications · 2026Article
- Atomic-level interface engineering enables efficient and durable acidic hydrogen evolution of osmium at large current densities.Chemical science · 2026Article
- Cerium driven active site relocation in spinel CoNature communications · 2026Article
- Ce Single Atom-Engineered Amorphous/Crystalline Nanosheets for Enhanced Alkaline Water Electrolysis.Advanced materials (Deerfield Beach, Fla.) · 2025Article
- Bioinspired Sulfo oxygen bridges optimize interfacial water structure for enhanced hydrogen oxidation and evolution reactions.Nature communications · 2025Article
- Atomically dispersed cerium on copper tailors interfacial water structure for efficient CO-to-acetate electroreduction.Nature communications · 2025Article
- Dominant Role of Coexisting Ruthenium Nanoclusters Over Single Atoms to Enhance Alkaline Hydrogen Evolution Reaction.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
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Authors and funding
13 authors.
Funding
Abstract
The state-of-the-art alkaline hydrogen evolution catalyst of united ruthenium single atoms and small ruthenium nanoparticles has sparked considerable research interest. However, it remains a serious problem that hydrogen evolution primarily proceeds on the less active ruthenium single atoms instead of the more efficient small ruthenium nanoparticles in the catalyst, hence largely falling short of its full activity potential. Here, we report that by combining highly oxophilic cerium single atoms and fully-exposed ruthenium nanoclusters on a nitrogen functionalized carbon support, the alkaline hydrogen evolution centers are facilely reversed to the more active ruthenium nanoclusters driven by the strong oxophilicity of cerium, which significantly improves the hydrogen evolution activity of the catalyst with its mass activity up to -10.1 A mg
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