Evidence map›Paper›PMID 38170817›Full record

ArticleThe Review of scientific instruments2024

A versatile pressure-cell design for studying ultrafast molecular-dynamics in supercritical fluids using coherent multi-pulse x-ray scattering.

Priyanka Muhunthan, Haoyuan Li, Guillaume Vignat, Edna R Toro, Khaled Younes, Yanwen Sun, Dimosthenis Sokaras, Thomas Weiss, Ivan Rajkovic, Taito Osaka and 6 more

Abstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in The Review of scientific instruments, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

16 authors.

Priyanka MuhunthanDepartment of Mechanical Engineering, Stanford University, Stanford, California 94305, USA.ORCID 0000-0001-9755-5245
Haoyuan LiDepartment of Mechanical Engineering, Stanford University, Stanford, California 94305, USA.ORCID 0000-0003-1845-3748
Guillaume VignatDepartment of Mechanical Engineering, Stanford University, Stanford, California 94305, USA.ORCID 0000-0002-5050-0009
Edna R ToroDepartment of Mechanical Engineering, Stanford University, Stanford, California 94305, USA.ORCID 0000-0002-8868-4325
Khaled YounesDepartment of Mechanical Engineering, Stanford University, Stanford, California 94305, USA.ORCID 0000-0001-9562-0963
Yanwen SunSLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.ORCID 0000-0001-5926-6565
Dimosthenis SokarasSLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.ORCID 0000-0001-8117-1933
Thomas WeissSLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.
Ivan RajkovicSLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.ORCID 0000-0003-4397-4801
Taito OsakaRIKEN SPring-8 Center, 1-1-1 Kouto, Sayo-cho, Sayo-gun, Hyogo 679-5148, Japan.
Ichiro InoueRIKEN SPring-8 Center, 1-1-1 Kouto, Sayo-cho, Sayo-gun, Hyogo 679-5148, Japan.ORCID 0009-0008-0423-1347
Sanghoon SongSLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.ORCID 0000-0003-3493-1850
Takahiro SatoSLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.ORCID 0000-0003-2202-0910
Diling ZhuSLAC National Accelerator Laboratory, Menlo Park, California 94025, USA.ORCID 0009-0001-4941-9799
John L FultonChemical and Materials Sciences Division, Pacific Northwest National Laboratory, Richland, Washington 99354, USA.ORCID 0000-0001-9361-9803
Matthias IhmeDepartment of Mechanical Engineering, Stanford University, Stanford, California 94305, USA.ORCID 0000-0002-4158-7050

Funding

A Synchrotron Radiation Structural Biology ResourcesP30GM133894 · NIGMS · STANFORD UNIVERSITY · PI Ritimukta Sarangi · 2020 to 2026
$43.3M
PILATUS3 X 1M X-ray detectorS10OD021512 · OD · STANFORD UNIVERSITY · PI WEIS, WILLIAM I · 2016 to 2016
$550k
NIGMS NIH HHS P30 GM133894NIH HHS S10 OD021512
6 · The paper itself

Abstract

Supercritical fluids (SCFs) can be found in a variety of environmental and industrial processes. They exhibit an anomalous thermodynamic behavior, which originates from their fluctuating heterogeneous micro-structure. Characterizing the dynamics of these fluids at high temperature and high pressure with nanometer spatial and picosecond temporal resolution has been very challenging. The advent of hard x-ray free electron lasers has enabled the development of novel multi-pulse ultrafast x-ray scattering techniques, such as x-ray photon correlation spectroscopy (XPCS) and x-ray pump x-ray probe (XPXP). These techniques offer new opportunities for resolving the ultrafast microscopic behavior in SCFs at unprecedented spatiotemporal resolution, unraveling the dynamics of their micro-structure. However, harnessing these capabilities requires a bespoke high-pressure and high-temperature sample system that is optimized to maximize signal intensity and address instrument-specific challenges, such as drift in beamline components, x-ray scattering background, and multi-x-ray-beam overlap. We present a pressure cell compatible with a wide range of SCFs with built-in optical access for XPCS and XPXP and discuss critical aspects of the pressure cell design, with a particular focus on the design optimization for XPCS.

Identifiers

PMID38170817
PMCPMC10771079

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.