ArticleNano letters2024
Electrochemically Switchable Multimode Strong Coupling in Plasmonic Nanocavities.
Article in Nano letters, 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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Who cites it
2 citing papers in PubMed.
- Collective multimode strong coupling in plasmonic nanocavities.Nanophotonics (Berlin, Germany) · 2025Article
- Active control of excitonic strong coupling and electroluminescence in electrically driven plasmonic nanocavities.Science advances · 2025Article
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Authors and funding
7 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The strong-coupling interaction between quantum emitters and cavities provides the archetypical platform for fundamental quantum electrodynamics. Here we show that methylene blue (MB) molecules interact coherently with subwavelength plasmonic nanocavity modes at room temperature. Experimental results show that the strong coupling can be switched on and off reversibly when MB molecules undergo redox reactions which transform them to leuco-methylene blue molecules. In simulations we demonstrate the strong coupling between the second excited plasmonic cavity mode and resonant emitters. However, we also show that other detuned modes simultaneously couple efficiently to the molecular transitions, creating unusual cascades of mode spectral shifts and polariton formation. This is possible due to the relatively large plasmonic particle size resulting in reduced mode splittings. The results open significant potential for device applications utilizing active control of strong coupling.
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