Evidence map›Paper›PMID 38110430›Full record

ArticleNature communications2023

Asynchronous domain dynamics and equilibration in layered oxide battery cathode.

Zhichen Xue, Nikhil Sharma, Feixiang Wu, Piero Pianetta, Feng Lin, Luxi Li, Kejie Zhao, Yijin Liu

Abstract read
In one paragraph

Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.

0numbers the graph read from it
0cells of the map it votes in
7citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

7 citing papers in PubMed.

  1. Review
  2. Article
  3. Chemical heterogeneity for battery materials.Nature reviews. Chemistry · 2026
    Review
  4. Review
  5. Article
  6. Review
  7. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

8 authors.

Zhichen XueSchool of Metallurgy and Environment, Central South University, 410083, Changsha, China.
Nikhil SharmaSchool of Mechanical Engineering, Purdue University, West Lafayette, IN, 47906, USA.ORCID http://orcid.org/0000-0002-6441-8452
Feixiang WuSchool of Metallurgy and Environment, Central South University, 410083, Changsha, China. feixiang.wu@csu.edu.cn.ORCID http://orcid.org/0000-0002-9688-2428
Piero PianettaStanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA, 94025, USA.ORCID http://orcid.org/0000-0002-4834-6014
Feng LinDepartment of Chemistry, Virginia Tech, Blacksburg, VA, 24061, USA.ORCID http://orcid.org/0000-0002-3729-3148
Luxi LiX-ray Science Division, Argonne National Laboratory, Lemont, IL, 60439, USA. luxili@anl.gov.ORCID http://orcid.org/0000-0002-9259-8796
Kejie ZhaoSchool of Mechanical Engineering, Purdue University, West Lafayette, IN, 47906, USA. kjzhao@purdue.edu.ORCID http://orcid.org/0000-0001-5030-7412
Yijin LiuWalker Department of Mechanical Engineering, The University of Texas at Austin, Austin, TX, 78712, USA. liuyijin@utexas.edu.ORCID http://orcid.org/0000-0002-8417-2488

Funding

National Natural Science Foundation of China (National Science Foundation of China) 52172264
6 · The paper itself

Abstract

To improve lithium-ion battery technology, it is essential to probe and comprehend the microscopic dynamic processes that occur in a real-world composite electrode under operating conditions. The primary and secondary particles are the structural building blocks of battery cathode electrodes. Their dynamic inconsistency has profound but not well-understood impacts. In this research, we combine operando coherent multi-crystal diffraction and optical microscopy to examine the chemical dynamics in local domains of layered oxide cathode. Our results not only pinpoint the asynchronicity of the lithium (de)intercalation at the sub-particle level, but also reveal sophisticated diffusion kinetics and reaction patterns, involving various localized processes, e.g., chemical onset, reaction front propagation, domains equilibration, particle deformation and motion. These observations shed new lights onto the activation and degradation mechanisms of state-of-the-art battery cathode materials.

Identifiers

PMID38110430
PMCPMC10728132

What OpenQuestion holds

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.