ArticleNano-micro letters2023
Exploring the Cation Regulation Mechanism for Interfacial Water Involved in the Hydrogen Evolution Reaction by In Situ Raman Spectroscopy.
Article in Nano-micro letters, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed, 67 citations in OpenAlex.
- Crystal Phase Engineering Accelerates Hydrogen Reverse Spillover for Efficient Alkaline Hydrogen Production.Nano-micro letters · 2026Article
- Hydrophobicity Modulated Interfacial Water Distribution for Enhanced Kinetics of HER.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Sulfur-engineered rhenium single-atoms on borides for tunable syngas and lactic acid co-production.Nature communications · 2026Article
- Engineering the interfacial water microenvironment to accelerate proton transfer for acidic oxygen evolution at high-potential.Chemical science · 2026Article
- Chelation-Buffer Co-Additives Enable Compact Zn Deposition and High-Rate Cycling in Zn-BrACS applied materials & interfaces · 2026Article
- Threefold-Hierarchical Transport of Highly Concentrated Aqueous Electrolyte Mediated by Environment-Reconstructed Ion Correlation Networks.Nano-micro letters · 2026Article
- Pulsed Dynamic Water Electrolysis: Mass Transfer Enhancement, Microenvironment Regulation, and Hydrogen Production Optimization.Nano-micro letters · 2026Review
- Entropy-driven difference in interfacial water reactivity between slab and nanodroplet.Nature communications · 2025Article
- Kinetic cation effect in alkaline hydrogen electrocatalysis and double layer proton transfer.Nature communications · 2025Article
- Accelerating Oxygen Electrocatalysis Kinetics on Metal-Organic Frameworks via Bond Length Optimization.Nano-micro letters · 2024Article
Corrections and comments
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Authors and funding
7 authors at 5 institutions in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Interfacial water molecules are the most important participants in the hydrogen evolution reaction (HER). Hence, understanding the behavior and role that interfacial water plays will ultimately reveal the HER mechanism. Unfortunately, investigating interfacial water is extremely challenging owing to the interference caused by bulk water molecules and complexity of the interfacial environment. Here, the behaviors of interfacial water in different cationic electrolytes on Pd surfaces were investigated by the electrochemistry, in situ core-shell nanostructure enhanced Raman spectroscopy and theoretical simulation techniques. Direct spectral evidence reveals a red shift in the frequency and a decrease in the intensity of interfacial water as the potential is shifted in the positively direction. When comparing the different cation electrolyte systems at a given potential, the frequency of the interfacial water peak increases in the specified order: Li
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