Evidence map›Paper›PMID 38103255›Full record

ArticleAngewandte Chemie (International ed. in English)2024

Probing Degradation in Lithium Ion Batteries with On-Chip Electrochemistry Mass Spectrometry.

Daisy B Thornton, Bethan J V Davies, Soren B Scott, Ainara Aguadero, Mary P Ryan, Ifan E L Stephens

Abstract read
In one paragraph

Article in Angewandte Chemie (International ed. in English), 2024. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.

0numbers the graph read from it
0cells of the map it votes in
2citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

2 citing papers in PubMed.

  1. Article
  2. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

6 authors.

Daisy B ThorntonDepartment of Materials, Imperial College London, London, SW7, UK.
Bethan J V DaviesDepartment of Materials, Imperial College London, London, SW7, UK.
Soren B ScottDepartment of Materials, Imperial College London, London, SW7, UK.
Ainara AguaderoDepartment of Materials, Imperial College London, London, SW7, UK.
Mary P RyanDepartment of Materials, Imperial College London, London, SW7, UK.
Ifan E L StephensDepartment of Materials, Imperial College London, London, SW7, UK.ORCID https://orcid.org/0000-0003-2157-492X

Funding

Armourers and BrasiersEngineering and Physical Sciences Research Council EP/S514901/1Faraday Institution FIRG024Fundación Iberdrola España Energy 4 FutureH2020 European Research Council 866402Henry Royce Institute EP/P02520X/1
6 · The paper itself

Abstract

The rapid uptake of lithium ion batteries (LIBs) for large scale electric vehicle and energy storage applications requires a deeper understanding of the degradation mechanisms. Capacity fade is due to the complex interplay between phase transitions, electrolyte decomposition and transition metal dissolution; many of these poorly understood parasitic reactions evolve gases as a side product. Here we present an on-chip electrochemistry mass spectrometry method that enables ultra-sensitive, fully quantified and time resolved detection of volatile species evolving from an operating LIB. The technique's electrochemical performance and mass transport is described by a finite element model and then experimentally used to demonstrate the variety of new insights into LIB performance. We show the versatility of the technique, including (a) observation of oxygen evolving from a LiNiMnCoO

Indexed as

DegradationElectrochemistryGas EvolutionLithium Ion BatteriesMass Spectrometry

Identifiers

PMID38103255
PMCPMC10962541

What OpenQuestion holds

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.