Evidence map›Paper›PMID 38100418›Full record

ArticleProceedings of the National Academy of Sciences of the United States of America2023

A polyimine aerogel separator with electron cloud design to boost Li-ion transport for stable Li metal batteries.

Luoyi Ding, Xinyang Yue, Xinhai Zhang, Yuanmao Chen, Jijiang Liu, Zhangqin Shi, Zhiyong Wang, Xuzhou Yan, Zheng Liang

Open access · hybridAbstract read
PubMed Full text at PMC Publisher
In one paragraph

Article in Proceedings of the National Academy of Sciences of the United States of America, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.

0numbers the graph read from it
0cells of the map it votes in
6citing papers in PubMed
5.5field-weighted citation impact, top 3% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

6 citing papers in PubMed, 42 citations in OpenAlex.

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4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

9 authors at 1 institution in 1 country.

Luoyi Ding *Frontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.
Xinyang Yue *Frontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.ORCID 0009-0005-8636-2575
Xinhai ZhangFrontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.ORCID 0000-0002-1604-6885
Yuanmao ChenFrontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.
Jijiang LiuFrontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.
Zhangqin ShiFrontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.
Zhiyong WangFrontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.
Xuzhou YanFrontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.ORCID 0000-0002-6114-5743
Zheng LiangFrontiers Science Center for Transformative Molecules, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, People's Republic of China.ORCID 0000-0001-9137-0338
Shanghai Jiao Tong University · CN

Funding

China Postdoctoral Science Foundation (China Postdoctoral Foundation Project) 2021M692061MOE | Fundamental Research Funds for the Central Universities (Fundamental Research Fund for the Central Universities) 22X010201631MOE | Fundamental Research Funds for the Central Universities (Fundamental Research Fund for the Central Universities) 23X010301599MOST | National Natural Science Foundation of China (NSFC) 22071152MOST | National Natural Science Foundation of China (NSFC) 22122105MOST | National Natural Science Foundation of China (NSFC) 22201177MOST | National Natural Science Foundation of China (NSFC) 52102282Starry Night Science Fund of Zhejiang University Shanghai Institute for Advanced Study SN-ZJU-SIAS-006STCSM | Natural Science Foundation of Shanghai Municipality () 20ZR1429200STCSM | Natural Science Foundation of Shanghai Municipality () 22dz1207603Young Elite Scientists Sponsorship Program by CAST 2020QNRC001
6 · The paper itself

Abstract

The separator with high Young's modulus can avoid the danger of large-sized dendrites, but regulating the chemical behavior of lithium (Li) at the separator/anode interface can effectively eliminate the dendrite issue. Herein, a polyimine aerogel (PIA) with accurate nitrogen (N) functional design is used as the functional separator in Li metal batteries to promote uniform Li nucleation and suppress the dendrite growth. Specifically, the imine (N1) and protonated tertiary amine (N2) sites in the molecular structure of the PIA are significantly different in electron cloud density (ECD) distribution. The N1 site with higher ECD and the N2 site with lower ECD tend to attract and repulse Li

Indexed as

covalent polymer networkLi-ion diffusionLi metal batterypolyimine aerogelseparator engineering

Identifiers

PMID38100418
PMCPMC10741384
OpenAlexW4389836966

What OpenQuestion holds

Textmetadata
LicenceCC BY-NC-ND
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.