ArticleChemical science2023
The magic of biaryl linkers: the electronic coupling through them defines the propensity for excited-state symmetry breaking in quadrupolar acceptor-donor-acceptor fluorophores.
Article in Chemical science, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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10 citing papers in PubMed.
- A unified solvatochromic-computational-machine-learning approach for solvent property prediction based on iodine color response.Chemical science · 2026Article
- In Silico Isomerization Produces Apt Negative Data for VHTS Validation.Journal of chemical information and modeling · 2026Article
- Article
- An efficient computational chemistry approach to generating negative data for drug discovery pipeline validation.Frontiers in bioinformatics · 2026Article
- Vibronic coupling-driven symmetry breaking and solvation in the photoexcited dynamics of quadrupolar dyes.Nature chemistry · 2025Article
- Tuning the Inter-Chromophore Electronic Coupling in Perylene Diimide Dimers with Rigid Covalent Linkers.Molecules (Basel, Switzerland) · 2025Article
- Computer-Generated, Mechanistic Networks Assist in Assigning the Outcomes of Complex Multicomponent Reactions.Journal of the American Chemical Society · 2025Article
- Shedding new light on quadrupolar 1,4-dihydropyrrolo[3,2-Chemical science · 2025Article
- 1,4-Dihydropyrrolo[3,2-The Journal of organic chemistry · 2025Article
- Strongly Polarized π-Extended 1,4-Dihydropyrrolo[3,2-The Journal of organic chemistry · 2024Article
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Authors and funding
10 authors.
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Abstract
Charge transfer (CT) is key for molecular photonics, governing the optical properties of chromophores comprising electron-rich and electron-deficient components. In photoexcited dyes with an acceptor-donor-acceptor or donor-acceptor-donor architecture, CT breaks their quadrupolar symmetry and yields dipolar structures manifesting pronounced solvatochromism. Herein, we explore the effects of electronic coupling through biaryl linkers on the excited-state symmetry breaking of such hybrid dyes composed of an electron-rich core,
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