Evidence map›Paper›PMID 38030620›Full record

ArticleNature communications2023

Unraveling the synergistic effects of Cu-Ag tandem catalysts during electrochemical CO

Marvin L Frisch, Longfei Wu, Clément Atlan, Zhe Ren, Madeleine Han, Rémi Tucoulou, Liang Liang, Jiasheng Lu, An Guo, Hong Nhan Nong and 5 more

Abstract read
In one paragraph

Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.

0numbers the graph read from it
0cells of the map it votes in
4citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

4 citing papers in PubMed.

  1. Article
  2. Article
  3. Review
  4. Local-strain-induced CONational science review · 2024
    Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

15 authors.

Marvin L Frisch *Department of Chemistry, Chemical Engineering Division, Technische Universitaet Berlin, Str. des 17. Juni 124, 10623, Berlin, Germany.ORCID http://orcid.org/0000-0001-5759-4020
Longfei Wu *Department of Chemistry, Chemical Engineering Division, Technische Universitaet Berlin, Str. des 17. Juni 124, 10623, Berlin, Germany.ORCID http://orcid.org/0000-0001-6330-3613
Clément AtlanESRF, The European Synchrotron, 71 Avenue des Martyrs, Grenoble, 38000, France.
Zhe RenDeutsches Elektronen-Synchrotron (DESY), Notkestr. 85, 22607, Hamburg, Germany.
Madeleine HanESRF, The European Synchrotron, 71 Avenue des Martyrs, Grenoble, 38000, France.
Rémi TucoulouESRF, The European Synchrotron, 71 Avenue des Martyrs, Grenoble, 38000, France.
Liang LiangDepartment of Chemistry, Chemical Engineering Division, Technische Universitaet Berlin, Str. des 17. Juni 124, 10623, Berlin, Germany.
Jiasheng LuDepartment of Chemistry, Chemical Engineering Division, Technische Universitaet Berlin, Str. des 17. Juni 124, 10623, Berlin, Germany.ORCID http://orcid.org/0000-0003-3283-1231
An GuoDepartment of Chemistry, Chemical Engineering Division, Technische Universitaet Berlin, Str. des 17. Juni 124, 10623, Berlin, Germany.
Hong Nhan NongDepartment of Chemistry, Chemical Engineering Division, Technische Universitaet Berlin, Str. des 17. Juni 124, 10623, Berlin, Germany.ORCID http://orcid.org/0000-0002-3192-3479
Aleks ArinchteinDepartment of Chemistry, Chemical Engineering Division, Technische Universitaet Berlin, Str. des 17. Juni 124, 10623, Berlin, Germany.
Michael SprungDeutsches Elektronen-Synchrotron (DESY), Notkestr. 85, 22607, Hamburg, Germany.ORCID http://orcid.org/0000-0003-2396-3304
Julie VillanovaESRF, The European Synchrotron, 71 Avenue des Martyrs, Grenoble, 38000, France.ORCID http://orcid.org/0000-0001-6157-2289
Marie-Ingrid RichardESRF, The European Synchrotron, 71 Avenue des Martyrs, Grenoble, 38000, France.ORCID http://orcid.org/0000-0002-8172-3141
Peter StrasserDepartment of Chemistry, Chemical Engineering Division, Technische Universitaet Berlin, Str. des 17. Juni 124, 10623, Berlin, Germany. pstrasser@tu-berlin.de.ORCID http://orcid.org/0000-0002-3884-436X

Funding

Bundesministerium für Bildung und Forschung (Federal Ministry of Education and Research) 03SF0611ADeutsche Forschungsgemeinschaft (German Research Foundation) STR 596/18-1Deutsche Forschungsgemeinschaft (German Research Foundation) STR 596/21-1EC | Horizon 2020 Framework Programme (EU Framework Programme for Research and Innovation H2020) 101006701EC | Horizon 2020 Framework Programme (EU Framework Programme for Research and Innovation H2020) 818823EC | Horizon 2020 Framework Programme (EU Framework Programme for Research and Innovation H2020) 851441
6 · The paper itself

Abstract

Controlling the selectivity of the electrocatalytic reduction of carbon dioxide into value-added chemicals continues to be a major challenge. Bulk and surface lattice strain in nanostructured electrocatalysts affect catalytic activity and selectivity. Here, we unravel the complex dynamics of synergistic lattice strain and stability effects of Cu-Ag tandem catalysts through a previously unexplored combination of in situ nanofocused X-ray absorption spectroscopy and Bragg coherent diffraction imaging. Three-dimensional strain maps reveal the lattice dynamics inside individual nanoparticles as a function of applied potential and product yields. Dynamic relations between strain, redox state, catalytic activity and selectivity are derived. Moderate Ag contents effectively reduce the competing evolution of H

Identifiers

PMID38030620
PMCPMC10687089

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.