Evidence map›Paper›PMID 38026812›Full record

ArticleACS catalysis2023

Bypassing Formation of Oxide Intermediate via Chemical Vapor Deposition for the Synthesis of an Mn-N-C Catalyst with Improved ORR Activity.

Thomas Stracensky, Li Jiao, Qiang Sun, Ershuai Liu, Fan Yang, Sichen Zhong, David A Cullen, Deborah J Myers, A Jeremy Kropf, Qingying Jia and 2 more

Abstract read
In one paragraph

Article in ACS catalysis, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 3 papers.

0numbers the graph read from it
0cells of the map it votes in
3citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

3 citing papers in PubMed.

  1. Review
  2. Article
  3. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

12 authors.

Thomas StracenskyDepartment of Chemistry and Chemical Biology, Northeastern University, Boston, Massachusetts 02115, United States.
Li JiaoDepartment of Chemical Engineering, Northeastern University, Boston, Massachusetts 02115, United States.
Qiang SunDepartment of Chemistry and Chemical Biology, Northeastern University, Boston, Massachusetts 02115, United States.
Ershuai LiuDepartment of Chemistry and Chemical Biology, Northeastern University, Boston, Massachusetts 02115, United States.ORCID https://orcid.org/0000-0002-6491-5504
Fan YangGiner, Inc, Newton, Massachusetts 02466, United States.
Sichen ZhongGiner, Inc, Newton, Massachusetts 02466, United States.
David A CullenCenter for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831, United States.ORCID https://orcid.org/0000-0002-2593-7866
Deborah J MyersChemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, Illinois 60439, United States.ORCID https://orcid.org/0000-0001-9299-3916
A Jeremy KropfChemical Sciences and Engineering Division, Argonne National Laboratory, Lemont, Illinois 60439, United States.ORCID https://orcid.org/0000-0002-3329-4493
Qingying JiaDepartment of Chemistry and Chemical Biology, Northeastern University, Boston, Massachusetts 02115, United States.
Sanjeev MukerjeeDepartment of Chemistry and Chemical Biology, Northeastern University, Boston, Massachusetts 02115, United States.ORCID https://orcid.org/0000-0002-2980-7655
Hui XuGiner, Inc, Newton, Massachusetts 02466, United States.

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

A significant barrier to the commercialization of proton exchange membrane fuel cells (PEMFCs) is the high cost of the platinum-based oxygen reduction reaction (ORR) cathode electrocatalysts. One viable solution is to replace platinum with a platinum-group metal (PGM) free catalyst with comparable activity and durability. However, PGM-free catalyst development is burdened by a lack of understanding of the active site formation mechanism during the requisite high-temperature synthesis step, thus making rational catalyst design challenging. Herein we demonstrate in-temperature X-ray absorption spectroscopy (XAS) to unravel the mechanism of site evolution during pyrolysis for a manganese-based catalyst. We show the transformation from an initial state of manganese oxides (MnO

Identifiers

PMID38026812
PMCPMC10660335

What OpenQuestion holds

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Registered trials

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.