ArticleNanoscale advances2023
Boosted ability of ZIF-8 for early-stage adsorption and degradation of chemical warfare agent simulants.
Article in Nanoscale advances, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Efficient adsorption of hazardous substances from the environment is crucial owing to the considerable risks they pose to both humans and ecosystems. Consequently, the development of porous materials with strong adsorption capabilities for hazardous substances, such as chemical warfare agents (CWAs), is pivotal for safeguarding human lives. Specifically, the early-stage adsorption proficiency of the adsorbents plays a vital role in determining their effectiveness as ideal adsorbents. Herein, we report the efficient adsorption of CWA simulants using thermally treated ZIF-8 (T-ZIF-8). The T-ZIF-8 samples were prepared by subjecting ZIF-8 to a simple thermal treatment, which resulted in a more positive surface charge with extra open metal sites. Although the pore volume of T-ZIF-8 decreased after thermal treatment, the positive surface charge of T-ZIF-8 proved advantageous for the adsorption of the CWA simulants. As a result, the adsorption capacity of T-ZIF-8 for the CWA simulants improved compared to that of pure ZIF-8. Notably, T-ZIF-8 exhibited a remarkably enhanced adsorption ability in the early stage of exposure to the CWA simulants, possibly due to the effective polar interactions between T-ZIF-8 and the simulants
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