ArticleScience advances2023
Strain-induced crystallization and phase separation used for fabricating a tough and stiff slide-ring solid polymer electrolyte.
Article in Science advances, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 21 papers.
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Who cites it
21 citing papers in PubMed, 123 citations in OpenAlex.
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- A caddisfly larva case-mimicked gel polymer electrolyte with high toughness and enhanced ion transport for safe lithium metal batteries.Science advances · 2026Article
- Organic supramolecular assemblage-confined photoluminescence.Chemical science · 2026Review
- A persistent-range hydrogen-bonded gel polymer electrolyte enabling wide-temperature and recyclable lithium metal batteries.Science advances · 2026Article
- An Elastocaloric Polymer with Ultra-High Solid-State Cooling via Defect Engineering.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Unraveling positive deformation rate-elongation relationships in tough and highly stretchable ionogels under rapid deformation.Nature communications · 2025Article
- Stiff and Fracture-Resistant Ion Gels Enabled by Synergetic Physical Entanglement and Hydrogen Bonding.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Dual polarization in extended π-conjugated zwitterionic COF facilitates LiChemical science · 2025Article
- Delayed crystallization response-inspired waterborne polyurethane with high performance.Nature communications · 2025Article
- Slide-Crosslinked Polyrotaxane Topological Networks: Quasi-Solid Electrolyte for High-Voltage Lithium Metal Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Self-reinforcement in filled rubber via strain-induced crystallisation.Nature communications · 2025Article
- Topological Vulcanization Strategy for Elastomeric Electrolytes with Enhanced Mechanical and Electrochemical Properties for Advanced Lithium Metal Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Gradient Solvent Replacement-Mediated Formation of High-Strength Hydrogel-Forming Microneedle for Long-Term Drug Delivery.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Topologically-crosslinked hydrogels based on γ-cyclodextrins.Communications chemistry · 2025Review
- Ultrastrong eutectogels engineered via integrated mechanical training in molecular and structural engineering.Nature communications · 2025Article
- Revealing and reconstructing the 3D Li-ion transportation network for superionic poly(ethylene) oxide conductor.Nature communications · 2024Article
- Rapidly damping hydrogels engineered through molecular friction.Nature communications · 2024Article
- Filled Elastomers: Mechanistic and Physics-Driven Modeling and Applications as Smart Materials.Polymers · 2024Review
Corrections and comments
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Authors and funding
6 authors at 3 institutions in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The demand for mechanically robust polymer-based electrolytes is increasing for applications to wearable devices. Young's modulus and breaking energy are essential parameters for describing the mechanical reliability of electrolytes. The former plays a vital role in suppressing the short circuit during charge-discharge, while the latter indicates crack propagation resistance. However, polymer electrolytes with high Young's moduli are generally brittle. In this study, a tough slide-ring solid polymer electrolyte (SR-SPE) breaking through this trade-off between stiffness and toughness is designed on the basis of strain-induced crystallization (SIC) and phase separation. SIC makes the material highly tough (breaking energy, 80 to 100 megajoules per cubic meter). Phase separation in the polymer enhanced stiffness (Young's modulus, 10 to 70 megapascals). The combined effect of phase separation and SIC made SR-SPE tough and stiff, while these mechanisms do not impair ionic conductivity. This SIC strategy could be combined with other toughening mechanisms to design tough polymer gel materials.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.