Evidence map›Paper›PMID 37992169›Full record

ArticleScience advances2023

Time-resolving state-specific molecular dissociation with XUV broadband absorption spectroscopy.

Alexander Magunia, Marc Rebholz, Elisa Appi, Christina C Papadopoulou, Hannes Lindenblatt, Florian Trost, Severin Meister, Thomas Ding, Michael Straub, Gergana D Borisova and 25 more

Abstract read
In one paragraph

Article in Science advances, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.

0numbers the graph read from it
0cells of the map it votes in
1citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

1 citing paper in PubMed.

  1. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

35 authors.

Alexander MaguniaMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0002-0969-9976
Marc RebholzMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0002-0035-1412
Elisa AppiLeibniz University Hannover, Welfengarten 1, 30167 Hannover, Germany.ORCID 0000-0003-3628-3543
Christina C PapadopoulouDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0002-3343-6981
Hannes LindenblattMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0003-1728-7979
Florian TrostMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0001-7756-286X
Severin MeisterMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0002-5245-8377
Thomas DingMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
Michael StraubMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0002-4698-0150
Gergana D BorisovaMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
Junhee LeeMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0009-0008-4985-9146
Rui JinMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
Alexander von der DellenMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
Christian KaiserMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.
Markus BrauneDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0002-2091-4585
Stefan DüstererDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0003-4379-1327
Skirmantas AlišauskasDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0002-7033-4087
Tino LangDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.
Christoph HeylDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0003-2133-5224
Bastian ManschwetusDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0001-6165-9560
Sören GrunewaldDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.
Ulrike FrühlingDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0002-8423-786X
Ayhan TajalliDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.
Ammar Bin WahidCenter for Free-Electron Laser Science (CFEL), Deutsches Elektronen-Synchrotron (DESY), Notkestr. 85, 22607 Hamburg, Germany.ORCID 0000-0003-0460-7072
Laura SillettiCenter for Free-Electron Laser Science (CFEL), Deutsches Elektronen-Synchrotron (DESY), Notkestr. 85, 22607 Hamburg, Germany.
Francesca CalegariCenter for Free-Electron Laser Science (CFEL), Deutsches Elektronen-Synchrotron (DESY), Notkestr. 85, 22607 Hamburg, Germany.ORCID 0000-0003-3234-7298
Philip MoselLeibniz University Hannover, Welfengarten 1, 30167 Hannover, Germany.
Uwe MorgnerLeibniz University Hannover, Welfengarten 1, 30167 Hannover, Germany.ORCID 0000-0001-5103-9632
Milutin KovacevLeibniz University Hannover, Welfengarten 1, 30167 Hannover, Germany.
Uwe ThummJ. R. Macdonald Laboratory, Kansas State University, Manhattan, KS 66506,USA.ORCID 0000-0001-9378-6601
Ingmar HartlDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0001-7274-754X
Rolf TreuschDeutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg, Germany.ORCID 0000-0001-8479-8862
Robert MoshammerMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0002-3666-4904
Christian OttMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0003-4110-0916
Thomas PfeiferMax-Planck-Institut für Kernphysik, Saupfercheckweg 1, 69117 Heidelberg, Germany.ORCID 0000-0002-5312-3747

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

The electronic and nuclear dynamics inside molecules are essential for chemical reactions, where different pathways typically unfold on ultrafast timescales. Extreme ultraviolet (XUV) light pulses generated by free-electron lasers (FELs) allow atomic-site and electronic-state selectivity, triggering specific molecular dynamics while providing femtosecond resolution. Yet, time-resolved experiments are either blind to neutral fragments or limited by the spectral bandwidth of FEL pulses. Here, we combine a broadband XUV probe pulse from high-order harmonic generation with an FEL pump pulse to observe dissociation pathways leading to fragments in different quantum states. We temporally resolve the dissociation of a specific O

Identifiers

PMID37992169
PMCPMC10664994

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Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.