ArticleProceedings of the National Academy of Sciences of the United States of America2023
Electrochemical interfacial catalysis in Co-based battery electrodes involving spin-polarized electron transfer.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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Who cites it
5 citing papers in PubMed.
- Achieving accelerated electrochemical kinetics in lithium-sulfur batteries by regulating the asymmetry factorNational science review · 2026Article
- Local Electron Spin-State Engineering at Fe Sites for Highly Reversible Sodium-Ion Batteries.Small methods · 2026Article
- Ligand engineering enhances (photo) electrocatalytic activity and stability of zeolitic imidazolate frameworks via in-situ surface reconstruction.Nature communications · 2024Article
- A fast-charging/discharging and long-term stable artificial electrode enabled by space charge storage mechanism.Nature communications · 2024Article
- Real-time tracking of electron transfer at catalytically active interfaces in lithium-ion batteries.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
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Authors and funding
12 authors.
Funding
Abstract
Interfacial catalysis occurs ubiquitously in electrochemical systems, such as batteries, fuel cells, and photocatalytic devices. Frequently, in such a system, the electrode material evolves dynamically at different operating voltages, and this electrochemically driven transformation usually dictates the catalytic reactivity of the material and ultimately the electrochemical performance of the device. Despite the importance of the process, comprehension of the underlying structural and compositional evolutions of the electrode material with direct visualization and quantification is still a significant challenge. In this work, we demonstrate a protocol for studying the dynamic evolution of the electrode material under electrochemical processes by integrating microscopic and spectroscopic analyses, operando magnetometry techniques, and density functional theory calculations. The presented methodology provides a real-time picture of the chemical, physical, and electronic structures of the material and its link to the electrochemical performance. Using Co(OH)
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Registered trials
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