ArticleThe journal of physical chemistry. C, Nanomaterials and interfaces2022
Water Adsorption on Mica Surfaces with Hydrophilicity Tuned by Counterion Types (Na, K, and Cs) and Structural Fluorination.
Article in The journal of physical chemistry. C, Nanomaterials and interfaces, 2022. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed, 14 citations in OpenAlex.
- Registry-Dependent Hydration in Layered Mineral Slit Pores: Insights from Molecular Simulations of Gibbsite and Muscovite.ACS omega · 2026Article
- Ion Distribution and Cation Exchange at Mica-Electrolyte Interfaces Probed with Deep Potential Molecular Dynamics.Chemistry of materials : a publication of the American Chemical Society · 2026Article
- Polymer-free van der Waals assembly of 2D material heterostructures using muscovite crystals.Nature communications · 2026Article
- Microstructure, Transport, and Mechanics of Compacted Clay Simulated at the 0.1 μm Scale (1400 Smectite Clay Particles) Using a Coarse-Grained Model with Explicit Counterions.The journal of physical chemistry. C, Nanomaterials and interfaces · 2026Article
- Using Static Multiple Light Scattering to Develop Microplastic-Free Seed Film-Coating Formulations.Molecules (Basel, Switzerland) · 2024Article
- Study on the Effect of Emulsifiers on the Properties of Oleogels Based on Olive Oil Containing Lidocaine.International journal of molecular sciences · 2024Article
- Hygroscopic Growth of Adsorbed Water Films on Smectite Clay Particles.Environmental science & technology · 2024Article
- Ion adsorption and hydration forces: a comparison of crystalline micaFaraday discussions · 2023Article
Corrections and comments
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Authors and funding
5 authors at 3 institutions in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The stability of adsorbed water films on mineral surfaces has far-reaching implications in the Earth, environmental, and materials sciences. Here, we use the basal plane of phlogopite mica, an atomically smooth surface of a natural mineral, to investigate water film structure and stability as a function of two features that modulate surface hydrophilicity: the type of adsorbed counterions (Na, K, and Cs) and the substitution of structural OH groups by F atoms. We use molecular dynamics simulations combined with in situ high-resolution X-ray reflectivity to examine surface hydration over a range of water loadings, from the adsorption of isolated water molecules to the formation of clusters and films. We identify four regimes characterized by distinct adsorption energetics and different sensitivities to cation type and mineral fluorination: from 0 to 0.5 monolayer film thickness, the hydration of adsorbed ions; from 0.5 to 1 monolayer, the hydration of uncharged regions of the siloxane surface; from 1 to 1.5 monolayer, the attachment of isolated water molecules on the surface of the first monolayer; and for >1.5 monolayer, the formation of an incipient electrical double layer at the mineral-water interface.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.