ArticleChemical science2023
Dielectric response of confined water films from a classical density functional theory perspective.
Article in Chemical science, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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Who cites it
1 citing paper in PubMed.
- Impedance of nanocapacitors from molecular simulations to understand the dynamics of confined electrolytes.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
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Authors and funding
4 authors.
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Abstract
We re-examine the problem of the dielectric response of highly polar liquids such as water in confinement between two walls using simple two-variable density functional theory involving number and polarisation densities. In the longitudinal polarisation case where a perturbing field is applied perpendicularly to the walls, we show that the notion of the local dielectric constant, although ill-defined at a microscopic level, makes sense when coarse-graining over the typical size of a particle is introduced. The approach makes it possible to study the effective dielectric response of thin liquid films of various thicknesses in connection with the recent experiments of Fumagalli
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