ArticleNature communications2023
Multi-scale molecular dynamics simulations of enhanced energy transfer in organic molecules under strong coupling.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 24 papers.
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Who cites it
24 citing papers in PubMed.
- Cavity-modified exciton-exciton annihilation in disordered molecular systems.Physical chemistry chemical physics : PCCP · 2026Article
- Quantum Dynamics Simulations of Polariton Transport in a Bloch Surface Wave Cavity.Nanophotonics (Berlin, Germany) · 2026Article
- Article
- Exciton-polariton dynamics in multilayered materials.Nature communications · 2026Article
- Interference-Induced Cavity Resonances and Imaginary Rabi Splitting.Nanophotonics (Berlin, Germany) · 2026Article
- Microscopic Theory of Polaron-Polariton Dispersion and Propagation.Nano letters · 2025Article
- Polaritonic quantum matter.Nanophotonics (Berlin, Germany) · 2025Review
- Perspective on Many-Body Methods for Molecular Polaritonic Systems.Journal of chemical theory and computation · 2025Review
- Impact of Dark Polariton States on Collective Strong Light-Matter Coupling in Molecules.The journal of physical chemistry letters · 2025Article
- Microscopic theory of polariton group velocity renormalization.Nature communications · 2025Article
- Disentangling Enhanced Diffusion and Ballistic Motion of Excitons Coupled to Bloch Surface Waves with Molecular Dynamics Simulations.The journal of physical chemistry letters · 2025Article
- Quantum dynamics simulation of exciton-polariton transport.Nature communications · 2025Article
- Radiative pumping vs vibrational relaxation of molecular polaritons: a bosonic mapping approach.Nature communications · 2025Article
- Cavity-enhanced energy transport in molecular systems.Nature materials · 2025Review
- Semiclassical Truncated-Wigner-Approximation Theory of Molecular Exciton-Polariton Dynamics in Optical Cavities.Journal of chemical theory and computation · 2025Article
- Mechanism of Molecular Polariton Decoherence in the Collective Light-Matter Couplings Regime.The journal of physical chemistry letters · 2024Article
- Condensation of Exciton-Polaritons in a Bound State in the Continuum: Effects of the Excitation Spot Size and Polariton Transport.ACS nano · 2024Article
- Thermal disorder prevents the suppression of ultra-fast photochemistry in the strong light-matter coupling regime.Nature communications · 2024Article
- Spatially Resolved Near Field Spectroscopy of Vibrational Polaritons at the Small N Limit.ACS photonics · 2024Article
- Coherent transient exciton transport in disordered polaritonic wires.Nanophotonics (Berlin, Germany) · 2024Article
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Authors and funding
5 authors.
Funding
Abstract
Exciton transport can be enhanced in the strong coupling regime where excitons hybridize with confined light modes to form polaritons. Because polaritons have group velocity, their propagation should be ballistic and long-ranged. However, experiments indicate that organic polaritons propagate in a diffusive manner and more slowly than their group velocity. Here, we resolve this controversy by means of molecular dynamics simulations of Rhodamine molecules in a Fabry-Pérot cavity. Our results suggest that polariton propagation is limited by the cavity lifetime and appears diffusive due to reversible population transfers between polaritonic states that propagate ballistically at their group velocity, and dark states that are stationary. Furthermore, because long-lived dark states transiently trap the excitation, propagation is observed on timescales beyond the intrinsic polariton lifetime. These insights not only help to better understand and interpret experimental observations, but also pave the way towards rational design of molecule-cavity systems for coherent exciton transport.
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