ArticleProceedings of the National Academy of Sciences of the United States of America2023
Slow-release synthesis of Cu single-atom catalysts with the optimized geometric structure and density of state distribution for Fenton-like catalysis.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
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Who cites it
12 citing papers in PubMed.
- Self-reconstruction of single copper atoms drives precise hydroxyl radicals generation for efficient water disinfection.Nature communications · 2026Article
- Single-Atom Iron Sites Enable Enhanced Arsenic Removal From Water Through Synergistic Adsorption-Oxidation.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Single-Atom Catalysts in Heterogeneous Electro-Fenton for Water Treatment: Design, Stability, and Applications.Chemistry, an Asian journal · 2026Review
- Dual-site single-atom catalysts achieve directional adsorption-oxidation control for enhanced photo-Fenton-like reactions.Nature communications · 2026Article
- Ultrafast energy-neutral molecular oxygen activation via atomically-adjacent bimetallic catalytic sites.Nature communications · 2025Article
- Anchoring Unimolecular Metal Chloride as a Sterically Active Site for Conformal Zinc Electrodeposition.Advanced materials (Deerfield Beach, Fla.) · 2025Article
- Single Atom Engineering for Electrocatalysis: Fundamentals and Applications.ACS catalysis · 2025Review
- Non-Aqueous Electrochemical COSmall (Weinheim an der Bergstrasse, Germany) · 2025Article
- Long-range interactions driving neighboring Fe-NNature communications · 2024Article
- Tuning electronic structure of metal-free dual-site catalyst enables exclusive singlet oxygen production and in-situ utilization.Nature communications · 2024Article
- Nanoconfinement steers nonradical pathway transition in single atom fenton-like catalysis for improving oxidant utilization.Nature communications · 2024Article
- Fenton-like activity and pathway modulation via single-atom sites and pollutants comediates the electron transfer process.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
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Authors and funding
6 authors.
Funding
Abstract
Single-atom Fenton-like catalysis has attracted significant attention, yet the quest for controllable synthesis of single-atom catalysts (SACs) with modulation of electron configuration is driven by the current disadvantages of poor activity, low selectivity, narrow pH range, and ambiguous structure-performance relationship. Herein, we devised an innovative strategy, the slow-release synthesis, to fabricate superior Cu SACs by facilitating the dynamic equilibrium between metal precursor supply and anchoring site formation. In this strategy, the dynamics of anchoring site formation, metal precursor release, and their binding reaction kinetics were regulated. Bolstered by harmoniously aligned dynamics, the selective and specific monatomic binding reactions were ensured to refine controllable SACs synthesis with well-defined structure-reactivity relationship. A copious quantity of monatomic dispersed metal became deposited on the C
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