ArticleChemistry of materials : a publication of the American Chemical Society2023
Synthesis of High Entropy and Entropy-Stabilized Metal Sulfides and Their Evaluation as Hydrogen Evolution Electrocatalysts.
Article in Chemistry of materials : a publication of the American Chemical Society, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 10 papers.
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Who cites it
10 citing papers in PubMed, 42 citations in OpenAlex.
- Pyrite High-Entropy Sulfides for Bifunctional Oxygen Electrocatalysis and High-Performance Zinc-Air Batteries.ACS omega · 2026Article
- Synthesis of rare earth doped MoSScientific reports · 2026Article
- Bringing Order to Chaos in High-Entropy Electrocatalysts.ACS energy letters · 2026Review
- Cu²⁺ as a dynamic director for Ce-incorporated (CoFeNiCuCe)₉S₈ nanoballs for multifunctional electrocatalysis.Communications chemistry · 2026Article
- Advanced materials for high-performance electrochemical water-splitting: a review of recent breakthroughs, and future prospects.Frontiers in chemistry · 2026Review
- Toward 2D van der Waals Entropy Mixture MXACS applied materials & interfaces · 2025Article
- Improving CO Oxidation Catalysis Over High Entropy Spinels by Increasing Disorder.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Using high pressure to investigate the stability of a high entropy wurtzite structured (MnFeCuAgZnCd)S.Communications chemistry · 2025Article
- A review of high-entropy materials with their unique applications.Advanced composites and hybrid materials · 2025Review
- Opportunities and Challenges in the Synthesis of Noble Metal Nanoparticles via the Chemical Route in Microreactor Systems.Micromachines · 2024Review
Corrections and comments
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Authors and funding
14 authors at 1 institution in 2 countries.
Funding
No grant is acknowledged in the PubMed record.
Abstract
High entropy metal chalcogenides are materials containing five or more elements within a disordered sublattice. These materials exploit a high configurational entropy to stabilize their crystal structure and have recently become an area of significant interest for renewable energy applications such as electrocatalysis and thermoelectrics. Herein, we report the synthesis of bulk particulate HE zinc sulfide analogues containing four, five, and seven metals. This was achieved using a molecular precursor cocktail approach with both transition and main group metal dithiocarbamate complexes which are decomposed simultaneously in a rapid (1 h) and low-temperature (500 °C) thermolysis reaction to yield high entropy and entropy-stabilized metal sulfides. The resulting materials were characterized by powder XRD, SEM, and TEM, alongside EDX spectroscopy at both the micro- and nano-scales. The entropy-stabilized (CuAgZnCoMnInGa)S material was demonstrated to be an excellent electrocatalyst for the hydrogen evolution reaction when combined with conducting carbon black, achieving a low onset overpotential of (∼80 mV) and η
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Registered trials
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