ArticleThe journal of physical chemistry letters2023
Does Coherence Affect the Multielectron Oxygen Reduction Reaction?
Article in The journal of physical chemistry letters, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.
What it found
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Who cites it
11 citing papers in PubMed.
- Chiral N-Heterocyclic Carbene On-Surface Induced Electronic Spin Filtration.Journal of the American Chemical Society · 2026Article
- Chiral-Encoded Pt-Ir Surfaces as Apparent Spin Filter for Enhanced Oxygen Reduction.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Chirality-promoted photocatalysis: a strategic framework for advancing future dye degradation technologies.RSC advances · 2026Article
- What Does It Take for an Organic Closed Shell Molecule to Become Magnetic?The journal of physical chemistry letters · 2025Review
- Article
- Sevoflurane and Desflurane Spin-Decoherence Effect on Fe(III)acetylacetonate Redox Process.Molecules (Basel, Switzerland) · 2025Article
- Engineered chirality of one-dimensional nanowires.Science advances · 2025Article
- Chirality Assisted Triplet Electron Pairing.The journal of physical chemistry letters · 2025Article
- The chirality-induced spin selectivity effect in asymmetric spin transport: from solution to device applications.Chemical science · 2024Review
- A chemical perspective on the chiral induced spin selectivity effect.National science review · 2024Review
- Chiral Induced Spin Selectivity.Chemical reviews · 2024Review
Corrections and comments
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Authors and funding
7 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
The oxygen reduction reaction (ORR) is the key for oxygen-based respiration and the operation of fuel cells. It involves the transmission of two pairs of electrons. We probed what type of interaction between the electrons is required to enable their efficient transfer into the oxygen. We show experimentally that the transfer of the electrons is controlled by the "hidden property" and present a theoretical model suggesting that it is related to coherent phase relations between the two electrons. Using spin polarization electrochemical measurements, with electrodes coated with different thicknesses of chiral coating, we confirm the special relation between the electrons. This relation is destroyed by multiple scattering events that result in the formation of hydrogen peroxide, which indicates a reduction in the ORR efficiency. Another indication for the possible role of coherence is the fluctuations in the reaction efficiency as a function of thickness of the chiral coated electrode.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.