ArticleThe journal of physical chemistry. C, Nanomaterials and interfaces2023
Atomic-Level and Surface Structure of Calcium Silicate Hydrate Nanofoils.
Article in The journal of physical chemistry. C, Nanomaterials and interfaces, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
What it found
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The trial behind it
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Who cites it
7 citing papers in PubMed.
- Self-Assembly of Organic-Inorganic Copolymers Toward Bio-Inspired Cementitious Composites.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Article
- Effects and Mechanisms of Calcium Silicate Hydrate on Microstructure and Thermal Properties of Hybrid MTMS-Silica Aerogels.Gels (Basel, Switzerland) · 2026Article
- Immobilization of CaPhysical chemistry chemical physics : PCCP · 2026Article
- Exploring the aluminium paradox in calcium-aluminosilicate-hydrate decalcification.Nature communications · 2025Article
- Relevance of Specific Surface of Mixed Oxide Derived from Layered Double Hydroxides on the Rheological Properties and Porosity of Cement Pastes.ACS applied materials & interfaces · 2025Review
- Exploring the Potential of Nonclassical Crystallization Pathways to Advance Cementitious Materials.Chemical reviews · 2024Review
Corrections and comments
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Authors and funding
4 authors.
Funding
No grant is acknowledged in the PubMed record.
Abstract
Deciphering the calcium silicate hydrate (C-S-H) surface is crucial for unraveling the mechanisms of cement hydration and property development. Experimental observations of C-S-H in cement systems suggest a surface termination which is fundamentally different from the silicate-terminated surface assumed in many atomistic level studies. Here, a new multiparameter approach to describing the (001) basal C-S-H surface is developed, which considers how the surface termination affects the overall properties (Ca/Si ratio, mean chain length, relative concentration of silanol and hydroxide groups). Contrary to current beliefs, it is concluded that the (001) C-S-H surface is dominantly calcium terminated. Finally, an adsorption mechanism for calcium and hydroxide ions is proposed, which is in agreement with the surface charge densities observed in previous studies.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.