Evidence map›Paper›PMID 37751290›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2023

Interweaving Elastic and Hydrogen Bond-Forming Polymers into Highly Tough and Stress-Relaxable Binders for High-Performance Silicon Anode in Lithium-Ion Batteries.

Daun Jeong, Jinsol Yook, Da-Sol Kwon, Jimin Shim, Jong-Chan Lee

Abstract read
In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.

0numbers the graph read from it
0cells of the map it votes in
8citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

8 citing papers in PubMed.

  1. Article
  2. Review
  3. Article
  4. Article
  5. Structural Design and Challenges of Micron-Scale Silicon-Based Lithium-ion Batteries.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025
    Review
  6. Article
  7. Article
  8. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

5 authors.

Daun JeongEnergy Storage Research Center, Korea Institute of Science and Technology (KIST), 14 Gil 5 Hwarang-ro, Seongbuk-gu, Seoul, 02792, Republic of Korea.
Jinsol YookSchool of Chemical and Biological Engineering and Institute of Chemical Processes, Seoul National University, 1, Gwanak-ro, Gwanak-gu, Seoul, 08826, Republic of Korea.
Da-Sol KwonEnergy Storage Research Center, Korea Institute of Science and Technology (KIST), 14 Gil 5 Hwarang-ro, Seongbuk-gu, Seoul, 02792, Republic of Korea.
Jimin ShimEnergy Storage Research Center, Korea Institute of Science and Technology (KIST), 14 Gil 5 Hwarang-ro, Seongbuk-gu, Seoul, 02792, Republic of Korea.ORCID https://orcid.org/0000-0001-6147-921X
Jong-Chan LeeSchool of Chemical and Biological Engineering and Institute of Chemical Processes, Seoul National University, 1, Gwanak-ro, Gwanak-gu, Seoul, 08826, Republic of Korea.ORCID https://orcid.org/0000-0002-5587-1183

Funding

National Research Foundation of Korea 2018R1A5A1024127National Research Foundation of Korea 2020M3H4A3081889National Research Foundation of Korea 2021R1A2C2006243National Research Foundation of Korea 2022M3H4A1A03076498National Research Foundation of Korea RS-2023-00209631
6 · The paper itself

Abstract

A central challenge in practically using high-capacity silicon (Si) as anode materials for lithium-ion batteries is alleviating significant volume change of Si during cycling. One key to resolving the failure issues of Si is exploiting carefully designed polymer binders exhibiting mechanical robustness to retain the structural integrity of Si electrodes, while concurrently displaying elasticity and toughness to effectively dissipate external stresses exerted by the volume changes of Si. Herein, a highly elastic and tough polymer binder is proposed by interweaving polyacrylic acid (PAA) with poly(urea-urethane) (PUU) elastomer for Si anodes. By systematically tuning molecular parameters, including molecular weights of hard/soft segments and structures of hard segment components, it is demonstrated that the mechanical properties of polymer binders, such as elasticity, toughness, and stress relaxation ability, strongly affect the cycling performance of Si electrodes. This study provides new insight into the rational design of polymer binders capable of accommodating the volume changes of Si, primarily by judicious modulation of the mechanical properties of polymer binders.

Indexed as

binderselastic polymerslithium-ion batteriessilicon anodesstress relaxation

Identifiers

PMID37751290
PMCPMC10625081

What OpenQuestion holds

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LicenceCC BY
Read underepoch 390

Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.