ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2023
Construction of Thiadiazole-Linked Covalent Organic Frameworks via Facile Linkage Conversion with Superior Photocatalytic Properties.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 6 papers.
What it found
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Who cites it
6 citing papers in PubMed, 43 citations in OpenAlex.
- Rational Synthesis of Extended π-Conjugated Covalent Organic Frameworks for Enhanced Photocatalytic Uranium(VI) Removal.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Conjugation Lock-In Reinforced Sulfur-Heteropolycyclic Covalent Organic Frameworks with Asymmetric Electron Distribution for Photocatalytic Aerobic Oxidation Reactions.Journal of the American Chemical Society · 2026Article
- Defect Engineering Activates Pyrene-Based Covalent Organic Frameworks for Efficient Photocatalytic Uranium Capture.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Photons, Excitons, and Electrons in Covalent Organic Frameworks.Journal of the American Chemical Society · 2024Review
- Organic Donor-Acceptor Systems for Photocatalysis.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Review
- Construction of Thiadiazole-Linked Covalent Organic Frameworks via Facile Linkage Conversion with Superior Photocatalytic Properties.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
Corrections and comments
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Authors and funding
4 authors at 1 institution in 1 country.
Funding
Abstract
The establishment of facile synthetic routes to engineer covalent organic frameworks (COFs) with fully conjugated structure and excellent stability is highly desired for practical applications in optoelectronics and photocatalysis. Herein, a novel linkage conversion strategy is reported to prepare crystalline thiadiazole-linked COFs via thionation, cyclization, and oxidation of N-acylhydrazole bonds with Lawesson's reagent (LR). The as-prepared thiadiazole-linked COFs not only remain porosity and crystallinity, but enhance its chemical stability. Furthermore, thiadiazole-linked COFs are more favorable to lower exciton binding energy and promote π-electron delocalization over the whole reticular framework than N-acylhydrazone-linked COFs. Notably, the extended π-conjugation structure and decent crystallinity of the resulting TDA-COF are reflected by its higher photocatalytic H
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.