ArticleThe journal of physical chemistry letters2023
Experimental Access to Mode-Specific Coupling between Quantum Molecular Vibrations and Classical Bath Modes.
Article in The journal of physical chemistry letters, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 1 paper.
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3 authors.
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Abstract
The interaction of quantum-mechanical systems with a fluctuating thermal environment (bath) is fundamental to molecular mechanics and energy transport/dissipation. Its complete picture requires mode-specific measurements of this interaction and an understanding of its nature. Here, we present a combined experimental and theoretical study providing detailed insights into the coupling between a high-frequency vibrational two-level system and thermally excited terahertz modes. Experimentally, two-dimensional terahertz-infrared-visible spectroscopy reports directly on the coupling between quantum oscillators represented by CH
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