ArticleChemical science2023
Improving the molecular spin qubit performance in zirconium MOF composites by mechanochemical dilution and fullerene encapsulation.
Article in Chemical science, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Zr-based metal-organic frameworks for colorimetric sensing applications.RSC applied interfaces · 2026Review
- Enlarging Quantum Coherence of Vanadyl Spin Qubits in Zirconium Porphyrinic MOFs.Inorganic chemistry · 2026Article
- Orientationally Resolved Electron-Spin Relaxation and Coherence in Fullerene-Encapsulated Rare-Earth Dimers with a Single-Electron Metal-Metal Bond.Journal of the American Chemical Society · 2026Article
- Mechanochemistry for Metal-Organic Frameworks and Covalent-Organic Frameworks (MOFs, COFs): Methods, Materials, and Mechanisms.Advanced materials (Deerfield Beach, Fla.) · 2025Review
- A Triple-Site GdACS applied materials & interfaces · 2025Article
- Stable Unpaired Electron States in the Lu-Lu Bond Leading to the Absence of Odd-Even Parity in the Kondo Effect of LuNano letters · 2025Article
- Phononic modulation of spin-lattice relaxation in molecular qubit frameworks.Nature communications · 2024Article
- Recent advances in supramolecular fullerene chemistry.Chemical Society reviews · 2024Review
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Authors and funding
11 authors.
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Abstract
Enlarging the quantum coherence times and gaining control over quantum effects in real systems are fundamental for developing quantum technologies. Molecular electron spin qubits are particularly promising candidates for realizing quantum information processing due to their modularity and tunability. Still, there is a constant search for tools to increase their quantum coherence times. Here we present how the mechanochemical introduction of active spin qubits in the form of 10% diluted copper(ii)-porphyrins in the diamagnetic PCN-223 and MOF-525 zirconium-MOF polymorph pair can be achieved. Furthermore, the encapsulation of fullerene during the MOF synthesis directs the process exclusively toward the rare PCN-223 framework with a controllable amount of fullerene in the framework channels. In addition to the templating role, the incorporation of fullerene increases the electron spin-lattice and phase-memory relaxation times,
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