ArticleJournal of the American Chemical Society2023
Backbone Engineering of Monodisperse Conjugated Polymers via Integrated Iterative Binomial Synthesis.
Article in Journal of the American Chemical Society, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.
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5 citing papers in PubMed.
- Challenges and Opportunities for Cleavable Linkers Used in Polymer-Drug Conjugates.Journal of the American Chemical Society · 2026Review
- Topology-controlled dynamic conjugated oligomers from tetra-arylsubstituted alkene building blocks.Nature communications · 2026Article
- BidirectionalMacromolecules · 2025Article
- Expeditious chemical synthesis of xylomannans disproves the proposed antifreeze activities.National science review · 2024Article
- Iterative SuFEx approach for sequence-regulated oligosulfates and its extension to periodic copolymers.Nature communications · 2024Article
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5 authors.
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Abstract
Synthesis of sequence-defined monodisperse π-conjugated polymers with versatile backbones remains a substantial challenge. Here we report the development of an integrated iterative binomial synthesis (IIBS) strategy to enable backbone engineering of conjugated polymers with precisely controlled lengths and sequences as well as high molecular weights. The IIBS strategy capitalizes on the use of phenol as a surrogate for aryl bromide and represents the merge between protecting-group-aided iterative synthesis (PAIS) and iterative binomial synthesis (IBS). Long and monodisperse conjugated polymers with diverse irregular backbones, which are inaccessible by conventional polymerizations, can be efficiently prepared by IIBS. In addition, topology-dependent and chain-length-dependent properties have been investigated.
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