ArticleProceedings of the National Academy of Sciences of the United States of America2023
Correlated surface-charging behaviors of two electrodes in an electrochemical cell.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 4 papers.
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Who cites it
4 citing papers in PubMed.
- Deciphering multi-dimensional interfacial mechanisms via organic cosolvent engineering for sustainable zinc metal batteries.Nature communications · 2025Article
- Plasmonic in-situ imaging of zeta potential distributions at electrochemical interfaces of 2D materials in water.Nature communications · 2025Article
- Pure Water Splitting Driven by Overlapping Electric Double Layers.Journal of the American Chemical Society · 2024Article
- Theoretical framework for mixed-potential-driven catalysis.Communications chemistry · 2024Article
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Authors and funding
3 authors.
Funding
Abstract
It is revealed herein that surface-charging behaviors of the two electrodes constituting an electrochemical cell cannot be described independently by their respective electric double-layer (EDL) properties. Instead, they are correlated in such a way that the surface-charging behavior of each electrode is determined by the EDL and the reaction kinetics at both electrodes. Two fundamental equations describing the correlated surface-charging behaviors are derived, and approximate analytical solutions are obtained at low and high current densities, respectively, to facilitate transparent understanding. Important implications of the presented conceptual analysis for theoretical and computational electrochemistry are discussed. A strategy of modulating the activity of one electrode by tuning EDL parameters of the other in a two-electrode electrochemical cell is demonstrated.
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