ArticleNature communications2023
Theory predicts UV/vis-to-IR photonic down conversion mediated by excited state vibrational polaritons.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 7 papers.
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Who cites it
7 citing papers in PubMed, 10 citations in OpenAlex.
- Exciton-polariton dynamics in multilayered materials.Nature communications · 2026Article
- Ultrafast optical modulation of vibrational strong coupling in ReCl(CO)Nanophotonics (Berlin, Germany) · 2025Article
- Excited State Dynamics of COJournal of the American Chemical Society · 2025Article
- Quantum dynamics simulation of exciton-polariton transport.Nature communications · 2025Article
- On-demand heralded MIR single-photon source using a cascaded quantum system.Science advances · 2025Article
- Photothermal Synergistic Hydrogen Production via a Fly-Ash-made Interfacial Vaporific System.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Theory predicts UV/vis-to-IR photonic down conversion mediated by excited state vibrational polaritons.Nature communications · 2023Article
Corrections and comments
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Authors and funding
4 authors at 1 institution in 1 country.
Funding
No grant is acknowledged in the PubMed record.
Abstract
This work proposes a photophysical phenomenon whereby ultraviolet/visible (UV/vis) excitation of a molecule involving a Franck-Condon (FC) active vibration yields infrared (IR) emission by strong coupling to an optical cavity. The resulting UV/vis-to-IR photonic down conversion process is mediated by vibrational polaritons in the electronic excited state potential. It is shown that the formation of excited state vibrational polaritons (ESVP) via UV/vis excitation only involve vibrational modes with both a non-zero FC activity and IR activity in the excited state. Density functional theory calculations are used to identify 1-Pyreneacetic acid as a molecule with this property and the dynamics of ESVP are modeled. Overall, this work introduces an avenue of polariton chemistry where excited state dynamics are influenced by the formation of vibrational polaritons. Along with this, the UV/vis-to-IR photonic down conversion is potentially useful in both sensing excited state vibrations and quantum transduction schemes.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.