Evidence map›Paper›PMID 37544912›Full record

ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2023

Coordinative Stabilization of Single Bismuth Sites in a Carbon-Nitrogen Matrix to Generate Atom-Efficient Catalysts for Electrochemical Nitrate Reduction to Ammonia.

Wuyong Zhang, Shaoqi Zhan, Jie Xiao, Tristan Petit, Christopher Schlesiger, Maximilian Mellin, Jan P Hofmann, Tobias Heil, Riccarda Müller, Kerstin Leopold and 1 more

Open access · goldAbstract read
In one paragraph

Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 5 papers.

0numbers the graph read from it
0cells of the map it votes in
5citing papers in PubMed
2.2field-weighted citation impact, top 11% of its field
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

5 citing papers in PubMed, 36 citations in OpenAlex.

  1. Review
  2. Article
  3. Article
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  5. Article
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

11 authors at 8 institutions in 5 countries.

Wuyong ZhangKey Laboratory of Advanced Fuel Cells and Electrolyzers Technology of Zhejiang Province, Qianwan Institute of CNITECH, Ningbo Institute of Materials Technology and Engineering, Chinese Academy of Sciences, Ningbo, Zhejiang, 315201, P. R. China.
Shaoqi ZhanDepartment of Chemistry-BMC, Uppsala University, BMC Box 576, Uppsala, S-751 23, Sweden.
Jie XiaoHelmholtz-Zentrum Berlin für Materialien und Energie GmbH, Albert-Einstein-Straße 15, 12489, Berlin, Germany.
Tristan PetitHelmholtz-Zentrum Berlin für Materialien und Energie GmbH, Albert-Einstein-Straße 15, 12489, Berlin, Germany.
Christopher SchlesigerInstitute for Optics and Atomic Physics, Technische Universität Berlin, Hardenbergstr. 36, 10623, Berlin, Germany.
Maximilian MellinSurface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt, Otto-Berndt-Straße 3, 64287, Darmstadt, Germany.
Jan P HofmannSurface Science Laboratory, Department of Materials and Earth Sciences, Technical University of Darmstadt, Otto-Berndt-Straße 3, 64287, Darmstadt, Germany.
Tobias HeilMax Planck Institute of Colloids and Interfaces, Department of Colloid Chemistry, Am Mühlenberg 1, 14476, Potsdam, Germany.
Riccarda MüllerInstitute of Analytical and Bioanalytical Chemistry, Ulm University, Albert-Einstein-Allee 11, 89081, Ulm, Germany.
Kerstin LeopoldInstitute of Analytical and Bioanalytical Chemistry, Ulm University, Albert-Einstein-Allee 11, 89081, Ulm, Germany.
Martin OschatzCenter for Energy and Environmental Chemistry Jena (CEEC Jena), Institute for Technical Chemistry and Environmental Chemistry, Friedrich-Schiller-University Jena, Philosophenweg 7a, 07743, Jena, Germany.ORCID https://orcid.org/0000-0003-2377-1214
Helmholtz-Zentrum Berlin für Materialien und Energie · DETechnische Universität Darmstadt · DEUniversität Ulm · DEChinese Academy of Sciences · CNFriedrich Schiller University Jena · DEMax Planck Institute of Colloids and Interfaces · DETechnische Universität Berlin · DEUppsala University · SE

Funding

Deutsche Forschungsgemeinschaft EXC2008/1-390540038Deutsche Forschungsgemeinschaft TRR234CataLight-364549901Strategic Priority Research Program of the Chinese Academy of Sciences XDB0450401
6 · The paper itself

Abstract

Electrochemical nitrate reduction to ammonia powered by renewable electricity is not only a promising alternative to the established energy-intense and non-ecofriendly Haber-Bosch reaction for ammonia generation but also a future contributor to the ever-more important denitrification schemes. Nevertheless, this reaction is still impeded by the lack of understanding for the underlying reaction mechanism on the molecular scale which is necessary for the rational design of active, selective, and stable electrocatalysts. Herein, a novel single-site bismuth catalyst (Bi-N-C) for nitrate electroreduction is reported to produce ammonia with maximum Faradaic efficiency of 88.7% and at a high rate of 1.38 mg h

Indexed as

ammonia productionelectrocatalysisnitrate reduction reactionsingle-site catalysts

Identifiers

PMID37544912
PMCPMC10558634
OpenAlexW4385615291

What OpenQuestion holds

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Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.