ArticleHeliyon2023
Conversion and rate behavior of brown macroalgae in pyrolysis: Detailed effects of operating parameters.
Article in Heliyon, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Not yet cited in PubMed.
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Abstract
Non-catalytic pyrolysis of brown macroalgae (Padina sp.) was studied in a batch reactor at temperature ranges of 400-600 °C and 10-90 min reaction times on the product distribution and conversion rate behavior. The highest pyro-oil and pyro-gas yields were obtained at 600 °C, which reached 67 wt% and 27 wt%, respectively, when the reaction times were prolonged (30-90 min). In addition, the high reaction temperature resulted in more generations of heavy tar and a considerable enhancement in aromatization degree. N-aromatic groups and phenol were observed from pyro-oil at 500 °C and 600 °C, respectively. Tar yield increased with reaction temperature, reflecting an order of reaction greater than one for tar production. The rate constant of tar formation was found to be 0.0013/s at 400 °C; 0.0023/s at 500 °C; and 0.0033/s at 600 °C, respectively, with the reaction order being higher than one (1.25). These findings highlighted that the proposed model could be used to accurately predict the pyrolysis process's behavior.
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