ArticleProceedings of the National Academy of Sciences of the United States of America2023
Contact between water vapor and silicate surface causes abiotic formation of reactive oxygen species in an anoxic atmosphere.
Article in Proceedings of the National Academy of Sciences of the United States of America, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 12 papers.
What it found
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Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
12 citing papers in PubMed, 43 citations in OpenAlex.
- RNA-Iron complexes catalyse prebiotic oxygen generation.Communications chemistry · 2026Article
- Additive-Free Contact-Electro-Catalysis/Vacuum Ultraviolet System for Rapid Mitigation of Antimicrobial-Resistance-Associated Contaminants in Water.Research (Washington, D.C.) · 2026Article
- Size Dependent Uncatalyzed Sulfite Oxidation in Aqueous Microdroplets.Environmental science & technology · 2025Article
- Functionalised Mesoporous Silica Thin Films as ROS-Generating Antimicrobial Coatings.International journal of molecular sciences · 2025Article
- Strategies for Improving Contact-Electro-Catalytic Efficiency: A Review.Nanomaterials (Basel, Switzerland) · 2025Review
- Onsite ammonia synthesis from water vapor and nitrogen in the air.Science advances · 2024Article
- Adsorbed microdroplets are mobile at the nanoscale.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- Effect of Sol-Gel Silica Matrices on the Chemical Properties of Adsorbed/Entrapped Compounds.Gels (Basel, Switzerland) · 2024Review
- Microdroplets initiate organic-inorganic interactions and mass transfer in thermal hydrous geosystems.Nature communications · 2024Article
- Busting the myth of spontaneous formation of HChemical science · 2024Article
- Continuous ammonia synthesis from water and nitrogen via contact electrification.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
- As air relative humidity increases, infectivity of SARS-CoV-2 decreases within water droplets.QRB discovery · 2024Article
Corrections and comments
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Authors and funding
8 authors at 4 institutions in 2 countries.
Funding
Abstract
Spontaneous generation of reactive oxygen species (ROS) in aqueous microdroplets or at a water vapor-silicate interface is a new source of redox chemistry. However, such generation occurs with difficulty in liquid water having a large ionic strength. We report that ROS is spontaneously produced when water vapor contacts hydrogen-bonded hydroxyl groups on a silicate surface. The evolution of hydrogen-bonded species such as hydroxyl groups was investigated by using two-dimensional, time-resolved FT-IR spectroscopy. The participation of water vapor in ROS generation is confirmed by investigating the reaction of D
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.