ArticleNature communications2023
Potential-dependent transition of reaction mechanisms for oxygen evolution on layered double hydroxides.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 47 papers.
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Who cites it
47 citing papers in PubMed.
- Defect-Driven Accelerated Reconstruction of Metal-Organic Frameworks Toward High-Performance Anion Exchange Membrane Water Electrolysis.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Revealing Local Coordination-Modulated Oxygen Evolution Reactivity in High-Entropy Layered Double Hydroxides.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- Ultrahigh Density Ir Single-Atom Catalysts With Synergistic Ir-Ir Pairs for Efficient Acidic Oxygen Evolution.Angewandte Chemie (International ed. in English) · 2026Article
- Iron-Promoted Dynamic Reconstruction of Perovskite Fluorides Toward Oxygen Evolution Reaction.ChemSusChem · 2026Article
- Operando-Defined Amorphous Energy Materials for Electrochemical Energy Systems: From Structural Definition to Descriptor-Guided Design.Materials (Basel, Switzerland) · 2026Review
- In-Situ Ni Leaching Induced the Formation of Amorphous High-Entropy Layered Hydroxides for Boosting the Oxygen Evolution Reaction.Small (Weinheim an der Bergstrasse, Germany) · 2026Article
- The Nickel Age in Electrocatalytic Anodic Reactions.JACS Au · 2026Review
- Synthesis and Regulation Mechanism of High Entropy Layered Double Hydroxide Electrocatalyst.Small (Weinheim an der Bergstrasse, Germany) · 2026Review
- Constructing high-density active sites on hollow covalent organic polymers for efficient oxygen electrocatalysis.Nature communications · 2026Article
- Self-adhesive high-entropy oxide sub-nanowire monolithic electrocatalysts.Nature nanotechnology · 2026Article
- DSKO: Dancing through DFTB Parametrization.Journal of chemical theory and computation · 2026Article
- Alkaline electrocatalytic water oxidation by Fe-Ni nanostructures on porous turbostratic carbon with tailorable metal-metal active sites.Chemical science · 2026Article
- Decoding active sites in high-entropy catalysts via attention-enhanced model.Science advances · 2026Article
- Dual-Site Synergistic Mechanism via Single-Atom and Vacancy Drives Lattice Oxygen Activation in Layered Double Hydroxides.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Article
- Machine-learning-guided tungsten single atoms promote oxyhydroxides for noble-metal-free water electrolysis.Nature communications · 2026Article
- Enhancement Strategies in Transition Metal Oxides as Efficient Electrocatalysts for the Oxygen Evolution Reaction.Molecules (Basel, Switzerland) · 2026Review
- Direct and Indirect Effects of Fe-Incorporation in Nickel(oxy)hydroxide Materials for the Electrocatalytic Oxygen Evolution Reaction - Employing Constant pH/U Models for Deeper Insights.Chemistry (Weinheim an der Bergstrasse, Germany) · 2025Article
- Identifying Beneficial and Adverse CoAdvanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025Article
- Chromium Cation-Induced Self-Reconstruction of a Stable and High Performance Boride-derived Electrocatalyst for Oxygen Evolution Reaction.Small (Weinheim an der Bergstrasse, Germany) · 2025Article
- Iron and oxygen vacancies co-modulated adsorption evolution and lattice oxygen dual-path mechanism for water oxidation.Nature communications · 2025Article
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Authors and funding
3 authors.
Funding
Abstract
Oxygen evolution reaction (OER) is of crucial importance to sustainable energy and environmental engineering, and layered double hydroxides (LDHs) are among the most active catalysts for OER in alkaline conditions, but the reaction mechanism for OER on LDHs remains controversial. Distinctive types of reaction mechanisms have been proposed for the O-O coupling in OER, yet they compose a coupled reaction network with competing kinetics dependent on applied potentials. Herein, we combine grand-canonical methods and micro-kinetic modeling to unravel that the nature of dominant mechanism for OER on LDHs transitions among distinctive types as a function of applied potential, and this arises from the interplay among applied potential and competing kinetics in the coupled reaction network. The theory-predicted overpotentials, Tafel slopes, and findings are in agreement with the observations of experiments including isotope labelling. Thus, we establish a computational methodology to identify and elucidate the potential-dependent mechanisms for electrochemical reactions.
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