ArticleAdvanced science (Weinheim, Baden-Wurttemberg, Germany)2023
Carbon Vacancies Steer the Activity in Dual Ni Carbon Nitride Photocatalysis.
Article in Advanced science (Weinheim, Baden-Wurttemberg, Germany), 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 9 papers.
What it found
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The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.
The trial behind it
Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.
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Who cites it
9 citing papers in PubMed, 54 citations in OpenAlex.
- On the Structure and Redox Behavior of Ni and Cu Single Atoms Supported on Carbon Nitride.Angewandte Chemie (International ed. in English) · 2026Article
- An asymmetric photothermal platform for coupled seawater splitting and desalination.Nature communications · 2026Article
- Light-driven ammonia electrooxidation via carbon nitride-ruthenium molecular interfaces.Beilstein journal of nanotechnology · 2026Article
- Toward Reliable and Reproducible Research in Organic Photocatalysis by Carbon Nitride.ACS catalysis · 2025Review
- Photocatalytic C(spNature communications · 2025Article
- What Is to Be Expected from Heterogeneous Catalysis in the Pipeline to Circular Economy?ChemSusChem · 2025Review
- On the Tracks to "Smart" Single-Atom Catalysts.Journal of the American Chemical Society · 2025Review
- Outstanding COAdvanced science (Weinheim, Baden-Wurttemberg, Germany) · 2024Article
- Carbon Vacancies Steer the Activity in Dual Ni Carbon Nitride Photocatalysis.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2023Article
Corrections and comments
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Authors and funding
22 authors at 8 institutions in 5 countries.
Funding
Abstract
The manipulation of carbon nitride (CN) structures is one main avenue to enhance the activity of CN-based photocatalysts. Increasing the efficiency of photocatalytic heterogeneous materials is a critical step toward the realistic implementation of sustainable schemes for organic synthesis. However, limited knowledge of the structure/activity relationship in relation to subtle structural variations prevents a fully rational design of new photocatalytic materials, limiting practical applications. Here, the CN structure is engineered by means of a microwave treatment, and the structure of the material is shaped around its suitable functionality for Ni dual photocatalysis, with a resulting boosting of the reaction efficiency toward many CX (X = N, S, O) couplings. The combination of advanced characterization techniques and first-principle simulations reveals that this enhanced reactivity is due to the formation of carbon vacancies that evolve into triazole and imine N species able to suitably bind Ni complexes and harness highly efficient dual catalysis. The cost-effective microwave treatment proposed here appears as a versatile and sustainable approach to the design of CN-based photocatalysts for a wide range of industrially relevant organic synthetic reactions.
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Registered trials
Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.