Evidence map›Paper›PMID 37350822›Full record

ArticleChemical science2023

PET recycling under mild conditions

Shengbo Zhang, Yingying Xue, Yanfen Wu, Yu-Xiao Zhang, Ting Tan, Zhiqiang Niu

Abstract read
In one paragraph

Article in Chemical science, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 11 papers.

0numbers the graph read from it
0cells of the map it votes in
11citing papers in PubMed
–field-weighted citation impact
1 · What the graph read from it

What it found

Each row is one number read from the abstract, on the scale the paper reported it, with its interval. Left of the dashed line favours the treatment, right favours the comparator. Under each row is the sentence it came from. New to these charts? A ten-minute tutorial.

The abstract states no effect estimate the extractor could read, or names no intervention and outcome on the map, so this paper lights no cell and moves no belief. It is still indexed, cited and linked below.

2 · The registry

The trial behind it

Trials whose registry record cites this paper, or whose number appears in the abstract. A trial that started after this paper was published is citing it as background, not reporting it.

Neither the registry nor the abstract names a trial number. If this is a trial report, that itself is worth knowing.

3 · Its place in the literature

Who cites it

11 citing papers in PubMed.

  1. Article
  2. Article
  3. Article
  4. Article
  5. Article
  6. Breaking the Recycling Bottleneck of Thermosets via Bio-Tailoring Technology.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2025
    Article
  7. Article
  8. Article
  9. Article
  10. Review
  11. Review
4 · The record

Corrections and comments

PubMed lists nothing against this paper. Absence here is not a guarantee, only a check that was made.

5 · Who and what money

Authors and funding

6 authors.

Shengbo ZhangDepartment State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University Beijing 100084 China niuzq@tsinghua.edu.cn.
Yingying XueLaboratory of Theoretical and Computational Nanoscience, CAS Key Laboratory of Nanophotonic Materials and Devices, National Center for Nanoscience and Technology, Chinese Academy of Sciences Beijing 100190 China tant@nanoctr.cn.
Yanfen WuDepartment State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University Beijing 100084 China niuzq@tsinghua.edu.cn.
Yu-Xiao ZhangDepartment State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University Beijing 100084 China niuzq@tsinghua.edu.cn.ORCID https://orcid.org/0000-0002-9112-9947
Ting TanLaboratory of Theoretical and Computational Nanoscience, CAS Key Laboratory of Nanophotonic Materials and Devices, National Center for Nanoscience and Technology, Chinese Academy of Sciences Beijing 100190 China tant@nanoctr.cn.
Zhiqiang NiuDepartment State Key Laboratory of Chemical Engineering, Department of Chemical Engineering, Tsinghua University Beijing 100084 China niuzq@tsinghua.edu.cn.ORCID https://orcid.org/0000-0002-9122-4880

Funding

No grant is acknowledged in the PubMed record.

6 · The paper itself

Abstract

Catalytic depolymerization represents a promising approach for the closed-loop recycling of plastic wastes. Here, we report a knowledge-driven catalyst development for poly(ethylene terephthalate) (PET) recycling, which not only achieves more than 23-fold enhancement in specific activity but also reduces the alkali concentration by an order of magnitude compared with the conventional hydrolysis. Substituted binuclear zinc catalysts are developed to regulate biomimetic intramolecular PET hydrolysis. Hammett studies and density functional theory (DFT) calculations indicate that the substituents modify the charge densities of the active centers, and an optimal substituent should slightly increase the electron richness of the zinc sites to facilitate the formation of a six-membered ring intermediate. The understanding of the structure-activity relationship leads to an advanced catalyst with a specific activity of 778 ± 40 g

Identifiers

PMID37350822
PMCPMC10283487

What OpenQuestion holds

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Registered trials

None linked

Read under generation 80e0d062 · epoch 390. Bibliography from PubMed, PubMed Central and OpenAlex; grants from NIH RePORTER; trial links from ClinicalTrials.gov; estimates, votes and beliefs from the OpenQuestion graph.