ArticleThe journal of physical chemistry letters2023
Theoretical Analysis of Exciton Wave Packet Dynamics in Polaritonic Wires.
Article in The journal of physical chemistry letters, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed, 22 citations in OpenAlex.
- Disentangling Enhanced Diffusion and Ballistic Motion of Excitons Coupled to Bloch Surface Waves with Molecular Dynamics Simulations.The journal of physical chemistry letters · 2025Article
- Quantum dynamics simulation of exciton-polariton transport.Nature communications · 2025Article
- Cavity-enhanced energy transport in molecular systems.Nature materials · 2025Review
- Thermal disorder prevents the suppression of ultra-fast photochemistry in the strong light-matter coupling regime.Nature communications · 2024Article
- Photochemical initiation of polariton-mediated exciton propagation.Nanophotonics (Berlin, Germany) · 2024Article
- Coherent transient exciton transport in disordered polaritonic wires.Nanophotonics (Berlin, Germany) · 2024Article
- Theoretical formulation of chemical equilibrium under vibrational strong coupling.Nature communications · 2024Article
- Multi-scale molecular dynamics simulations of enhanced energy transfer in organic molecules under strong coupling.Nature communications · 2023Article
Corrections and comments
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Authors and funding
3 authors at 1 institution in 1 country.
Funding
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Abstract
We present a comprehensive study of the exciton wave packet evolution in disordered lossless polaritonic wires. Our simulations reveal signatures of ballistic, diffusive, and subdiffusive exciton dynamics under strong light-matter coupling and identify the typical time scales associated with the transitions between these qualitatively distinct transport phenomena. We determine optimal truncations of the matter and radiation subsystems required for generating reliable time-dependent data from computational simulations at an affordable cost. The time evolution of the photonic part of the wave function reveals that many cavity modes contribute to the dynamics in a nontrivial fashion. Hence, a sizable number of photon modes is needed to describe exciton propagation with a reasonable accuracy. We find and discuss an intriguingly common lack of dominance of the photon mode on resonance with matter in both the presence and absence of disorder. We discuss the implications of our investigations for the development of theoretical models and analysis of experiments where coherent intermolecular energy transport and static disorder play an important role.
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