ArticleMolecules (Basel, Switzerland)2023
Theoretical Description of Attosecond X-ray Absorption Spectroscopy of Frenkel Exciton Dynamics.
Article in Molecules (Basel, Switzerland), 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 2 papers.
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2 citing papers in PubMed.
- An exciting Approach to Theoretical Spectroscopy.Advanced science (Weinheim, Baden-Wurttemberg, Germany) · 2026Review
- Toward ultrafast soft x-ray spectroscopy of organic photovoltaic devices.Structural dynamics (Melville, N.Y.) · 2024Article
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3 authors.
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Abstract
Frenkel excitons are responsible for the transport of light energy in many molecular systems. Coherent electron dynamics govern the initial stage of Frenkel-exciton transfer. Capability to follow coherent exciton dynamics in real time will help to reveal their actual contribution to the efficiency of light-harvesting. Attosecond X-ray pulses are the tool with the necessary temporal resolution to resolve pure electronic processes with atomic sensitivity. We describe how attosecond X-ray pulses can probe coherent electronic processes during Frenkel-exciton transport in molecular aggregates. We analyze time-resolved absorption cross section taking broad spectral bandwidth of an attosecond pulse into account. We demonstrate that attosecond X-ray absorption spectra can reveal delocalization degree of coherent exciton transfer dynamics.
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