ArticleNature communications2023
Visualizing the multi-level assembly structures of conjugated molecular systems with chain-length dependent behavior.
Article in Nature communications, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 8 papers.
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Who cites it
8 citing papers in PubMed.
- Single-crystal-like polymer semiconductors via self-templated gradient assembly for ultrahigh charge carrier mobility.Nature materials · 2026Article
- A rubbery semiconducting heterojunction film for fully rubbery multiplexed near-infrared phototransistor arrays.Science advances · 2026Article
- Roles of π‑Conjugation and Intermolecular Interactions in Molecular Raman, Fluorescence, and Lifetime Spectroscopy.ACS omega · 2026Article
- Morphology-Dependent Percolation and Conductive Network Formation in Polymer Nanocomposites with Multi-Shaped Nanofillers.Nanomaterials (Basel, Switzerland) · 2025Article
- Cicada rib-inspired tough films through nanoconfined crystallization for use in acoustic transducers.Science advances · 2025Article
- Uncovering three-body competition of chain growth, degradation and re-aggregation for polyphenylacetylenes during solution polymerization.RSC advances · 2025Article
- On-site biosignal amplification using a single high-spin conjugated polymer.Nature communications · 2025Article
- Perpendicular crossing chains enable high mobility in a noncrystalline conjugated polymer.Proceedings of the National Academy of Sciences of the United States of America · 2024Article
Corrections and comments
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Authors and funding
15 authors.
Funding
Abstract
It remains challenging to understand the structural evolution of conjugated polymers from single chains to solvated aggregates and film microstructures, although it underpins the performance of optoelectrical devices fabricated via the mainstream solution processing method. With several ensemble visual measurements, here we unravel the morphological evolution process of a model system of isoindigo-based conjugated molecules, including the hidden molecular assembly pathways, the mesoscale network formation, and their unorthodox chain dependence. Short chains show rigid chain conformations forming discrete aggregates in solution, which further grow to form a highly ordered film that exhibits poor electrical performance. In contrast, long chains exhibit flexible chain conformations, creating interlinked aggregates networks in solution, which are directly imprinted into films, forming interconnective solid-state microstructure with excellent electrical performance. Visualizing multi-level assembly structures of conjugated molecules provides a deep understanding of the inheritance of assemblies from solution to solid-state, accelerating the optimization of device fabrication.
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Registered trials
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