ArticleAccounts of chemical research2023
Proton-Coupled Electron Transfer at the Surface of Polyoxovanadate-Alkoxide Clusters.
Article in Accounts of chemical research, 2023. The graph could read no effect estimate from its abstract, so it casts no vote on the map. Cited by 15 papers.
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Who cites it
15 citing papers in PubMed.
- Evidence for Site-Specific Tunneling in H Atom Uptake at the Surface of Polyoxovanadate-Alkoxides.JACS Au · 2026Article
- Pre-association enables visible-light induced proton-coupled electron-transfer in a titanium-functionalized polyoxotungstate.Chemical science · 2026Article
- Repositioning Proton and Electron Donors in a Family of Proton-Coupled Electron Transfer Mediators.Inorganic chemistry · 2026Article
- The Effect of Nanoparticle Structure on the Thermodynamics and Kinetics of Proton-Coupled Electron Transfer Reactions to V2O5.Journal of the American Chemical Society · 2026Article
- Unique Structural Features of Polyoxometalates for Efficient Alkaline Hydrogen-Evolution Reaction.ChemSusChem · 2026Review
- Ensemble Effects on Hydroxide Bond Dissociation Free Energies in Polyoxovanadate Clusters.The journal of physical chemistry. A · 2026Article
- Multisite Proton-Coupled Electron Transfer at a Keggin-Type Polyoxotungstate.Journal of the American Chemical Society · 2026Article
- Impact of Anionic Dopants on H Atom Uptake at Polyoxovanadate-Alkoxide Surfaces.Inorganic chemistry · 2025Article
- Redox-Active Ligands Permit Multielectron OJournal of the American Chemical Society · 2025Article
- Redox Self-Equilibration in Molecular Vanadium Oxide Mixtures Enables Multi-Electron Storage.Angewandte Chemie (International ed. in English) · 2025Article
- Trap States in Reduced Colloidal Titanium Dioxide Nanoparticles Have Different Proton Stoichiometries.ACS central science · 2024Article
- Electrochemically Determined and Structurally Justified Thermochemistry of H atom Transfer on Ti-Oxo Nodes of the Colloidal Metal-Organic Framework Ti-MIL-125.Journal of the American Chemical Society · 2024Article
- Vanadium Substitution Dictates H Atom Uptake at Lindqvist-type Polyoxotungstates.Inorganic chemistry · 2024Article
- Selective Hydrogenation of Azobenzene to Hydrazobenzene via Proton-Coupled Electron Transfer from a Polyoxotungstate Cluster.JACS Au · 2024Article
- Impact of Surface Ligand Identity and Density on the Thermodynamics of H Atom Uptake at Polyoxovanadate-Alkoxide Surfaces.Inorganic chemistry · 2024Article
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3 authors.
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No grant is acknowledged in the PubMed record.
Abstract
ConspectusProton-coupled electron transfer (PCET) is a fundamental process involved in all areas of chemistry, with relevance to biological transformations, catalysis, and emergent energy storage and conversion technologies. Early observations of PCET were reported by Meyer and co-workers in 1981 while investigating the proton dependence of reduction of a molecular ruthenium oxo complex. Since that time, this conceptual framework has grown to encompass an enormous scope of charge transfer and compensation reactions. In this Account, we will discuss ongoing efforts in the Matson Laboratory to understand the fundamental thermodynamics and kinetics of PCET processes at the surface of a series of Lindqvist-type polyoxovanadate clusters. This project aims to provide atomistic resolution of net H atom uptake and transfer at the surfaces of transition-metal oxide materials.First, we discuss our efforts aimed at understanding PCET at metal oxide surfaces using the Lindqvist-type polyoxovanadate-alkoxide (POV-alkoxide) cluster [
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